Wei-cai Zhang , Chao-wei Yang , Shu-yu Hu , Ya-wei Fang , Xiao-min Lin , Zhuo-hao Xie , Ming-tao Zheng , Ying-liang Liu , Ye-ru Liang
{"title":"制备具有高锂离子存储能力的多金属硫化物/碳复合材料的一锅法","authors":"Wei-cai Zhang , Chao-wei Yang , Shu-yu Hu , Ya-wei Fang , Xiao-min Lin , Zhuo-hao Xie , Ming-tao Zheng , Ying-liang Liu , Ye-ru Liang","doi":"10.1016/S1872-5805(23)60781-4","DOIUrl":null,"url":null,"abstract":"<div><p>Because of their high electrochemical activity, good structural stability, and abundant active sites, multi-metal sulfide/carbon (MMS/C) composites are of tremendous interest in diverse fields, including catalysis, energy, sensing, and environmental science. However, their cumbersome, inefficient, and environmentally unfriendly synthesis is hindering their practical application. We report a straightforward and universal method for their production which is based on homogeneous multi-phase interface engineering. The method has enabled the production of 14 different MMS/C composites, as examples, with well-organized composite structures, different components, and dense heterointerfaces. Because of their composition and structure, a typical composite has efficient, fast, and persistent lithium-ion storage. A ZnS-Co<sub>9</sub>S<sub>8</sub>/C composite anode showed a remarkable rate performance and an excellent capacity of 651 mAh·g<sup>−1</sup> at 0.1 A·g<sup>−1</sup> after 600 cycles. This work is expected to pave the way for the easy fabrication of MMS/C composites.</p></div>","PeriodicalId":19719,"journal":{"name":"New Carbon Materials","volume":"38 6","pages":"Pages 1080-1091"},"PeriodicalIF":5.7000,"publicationDate":"2023-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A one-pot method to prepare a multi-metal sulfide/carbon composite with a high lithium-ion storage capability\",\"authors\":\"Wei-cai Zhang , Chao-wei Yang , Shu-yu Hu , Ya-wei Fang , Xiao-min Lin , Zhuo-hao Xie , Ming-tao Zheng , Ying-liang Liu , Ye-ru Liang\",\"doi\":\"10.1016/S1872-5805(23)60781-4\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Because of their high electrochemical activity, good structural stability, and abundant active sites, multi-metal sulfide/carbon (MMS/C) composites are of tremendous interest in diverse fields, including catalysis, energy, sensing, and environmental science. However, their cumbersome, inefficient, and environmentally unfriendly synthesis is hindering their practical application. We report a straightforward and universal method for their production which is based on homogeneous multi-phase interface engineering. The method has enabled the production of 14 different MMS/C composites, as examples, with well-organized composite structures, different components, and dense heterointerfaces. Because of their composition and structure, a typical composite has efficient, fast, and persistent lithium-ion storage. A ZnS-Co<sub>9</sub>S<sub>8</sub>/C composite anode showed a remarkable rate performance and an excellent capacity of 651 mAh·g<sup>−1</sup> at 0.1 A·g<sup>−1</sup> after 600 cycles. This work is expected to pave the way for the easy fabrication of MMS/C composites.</p></div>\",\"PeriodicalId\":19719,\"journal\":{\"name\":\"New Carbon Materials\",\"volume\":\"38 6\",\"pages\":\"Pages 1080-1091\"},\"PeriodicalIF\":5.7000,\"publicationDate\":\"2023-12-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"New Carbon Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1872580523607814\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"Materials Science\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"New Carbon Materials","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1872580523607814","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Materials Science","Score":null,"Total":0}
A one-pot method to prepare a multi-metal sulfide/carbon composite with a high lithium-ion storage capability
Because of their high electrochemical activity, good structural stability, and abundant active sites, multi-metal sulfide/carbon (MMS/C) composites are of tremendous interest in diverse fields, including catalysis, energy, sensing, and environmental science. However, their cumbersome, inefficient, and environmentally unfriendly synthesis is hindering their practical application. We report a straightforward and universal method for their production which is based on homogeneous multi-phase interface engineering. The method has enabled the production of 14 different MMS/C composites, as examples, with well-organized composite structures, different components, and dense heterointerfaces. Because of their composition and structure, a typical composite has efficient, fast, and persistent lithium-ion storage. A ZnS-Co9S8/C composite anode showed a remarkable rate performance and an excellent capacity of 651 mAh·g−1 at 0.1 A·g−1 after 600 cycles. This work is expected to pave the way for the easy fabrication of MMS/C composites.
期刊介绍：
New Carbon Materials is a scholarly journal that publishes original research papers focusing on the physics, chemistry, and technology of organic substances that serve as precursors for creating carbonaceous solids with aromatic or tetrahedral bonding. The scope of materials covered by the journal extends from diamond and graphite to a variety of forms including chars, semicokes, mesophase substances, carbons, carbon fibers, carbynes, fullerenes, and carbon nanotubes. The journal's objective is to showcase the latest research findings and advancements in the areas of formation, structure, properties, behaviors, and technological applications of carbon materials. Additionally, the journal includes papers on the secondary production of new carbon and composite materials, such as carbon-carbon composites, derived from the aforementioned carbons. Research papers on organic substances will be considered for publication only if they have a direct relevance to the resulting carbon materials.
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