含碳修正的美国农业土壤活性氮排放的农业生态系统模型

IF 13.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Biochar Pub Date : 2023-11-09 DOI:10.1007/s42773-023-00271-5
Lina Luo, Daniel S. Cohan, Caroline A. Masiello, Taras E. Lychuk, Xiaodong Gao
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引用次数: 0

摘要

肥料密集型农业是活性氮(Nr)排放的主要来源,会损害气候、空气质量和人类健康。生物炭作为土壤改良剂研究已久,但其对Nr排放的影响尚未充分表征。最近,轻烃的热解被认为是氢燃料的一种来源,产生固体零价碳(ZVC)副产品,其对土壤排放的影响尚未得到测试。我们将碳修正算法纳入农业生态系统模型,以模拟生物炭或ZVC在美国应用后一年的排放变化。受精的土壤。我们的模拟预测,生物炭对Nr排放的影响差异很大(在5吨ha - 1施用下为- 17%至+ 27%,在20吨ha - 1施用下为- 38%至+ 18%),主要取决于硝化作用如何受到影响。低剂量生物炭应用(5吨公顷- 1)在75%的模拟农业区刺激了所有三种氮的排放,而高剂量应用(20吨公顷- 1)减轻了76%的模拟农业区的排放。施用20吨公顷−1的零价碳对氮排放的影响与施用5吨公顷−1的生物炭相似。如果在酸性土壤(pH <5.84)与低有机碳(<55.9 kg cha - 1)和无机氮(<101.5 kg N ha−1)含量。我们的模拟可以告知在哪些地方应用碳修正最有可能减轻Nr排放及其相关的不利影响。图形抽象
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Agroecosystem modeling of reactive nitrogen emissions from U.S. agricultural soils with carbon amendments

Agroecosystem modeling of reactive nitrogen emissions from U.S. agricultural soils with carbon amendments
Abstract Fertilizer-intensive agriculture is a leading source of reactive nitrogen (Nr) emissions that damage climate, air quality, and human health. Biochar has long been studied as a soil amendment, but its influence on Nr emissions remains insufficiently characterized. More recently, the pyrolysis of light hydrocarbons has been suggested as a source of hydrogen fuel, resulting in a solid zero-valent carbon (ZVC) byproduct whose impact on soil emissions has yet to be tested. We incorporate carbon amendment algorithms into an agroecosystem model to simulate emission changes in the year following the application of biochar or ZVC to the US. fertilized soils. Our simulations predicted that the impacts of biochar amendments on Nr emissions would vary widely (− 17% to + 27% under 5 ton ha −1 applications, − 38% to + 18% under 20 ton ha −1 applications) and depend mostly on how nitrification is affected. Low-dose biochar application (5 ton ha −1 ) stimulated emissions of all three nitrogen species in 75% of simulated agricultural areas, while high-dose applications (20 ton ha −1 ) mitigated emissions in 76% of simulated areas. Applying zero-valent carbon at 20 ton ha −1 exhibited similar effects on nitrogen emissions as biochar applications at 5 ton ha −1 . Biochar amendments are most likely to mitigate emissions if applied at high rates in acidic soils (pH < 5.84) with low organic carbon (< 55.9 kg C ha −1 ) and inorganic nitrogen (< 101.5 kg N ha −1 ) content. Our simulations could inform where the application of carbon amendments would most likely mitigate Nr emissions and their associated adverse impacts. Graphical Abstract
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来源期刊
Biochar
Biochar Multiple-
CiteScore
18.60
自引率
10.20%
发文量
61
期刊介绍: Biochar stands as a distinguished academic journal delving into multidisciplinary subjects such as agronomy, environmental science, and materials science. Its pages showcase innovative articles spanning the preparation and processing of biochar, exploring its diverse applications, including but not limited to bioenergy production, biochar-based materials for environmental use, soil enhancement, climate change mitigation, contaminated-environment remediation, water purification, new analytical techniques, life cycle assessment, and crucially, rural and regional development. Biochar publishes various article types, including reviews, original research, rapid reports, commentaries, and perspectives, with the overarching goal of reporting significant research achievements, critical reviews fostering a deeper mechanistic understanding of the science, and facilitating academic exchange to drive scientific and technological development.
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