等离子体纳米壳附近的分子间能量传递

M. S. Shishodia, Soniya Juneja, B. Fainberg, A. Nitzan
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引用次数: 2

摘要

本文提出了一种新的理论方法,用于处理纳米壳附近供体和受体分子之间的能量转移相互作用。基于等离子体纳米壳的多种应用和丰富的等离子体特性,如表面等离子体频率的调谐能力、对介电环境的更高灵敏度和电磁辐射的可控重定向,推导了纳米壳介导的分子间能量转移放大因子的封闭表达式。本文导出的封闭形式表达式可直接用作公式;设计基于SP的生物传感器,计算量子点(QDs)中蛋白质之间的能量交换和激子相互作用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Intermolecular energy transfer near plasmonic nanoshell
A novel theoretical approach is developed for treating energy transfer interactions between a donor and an acceptor molecule in the proximity of a nanoshell. Motivated from the diverse applications and rich plasmonic features of plasmonic nanoshell for example, tuning capability of Surface Plasmon (SP) frequencies, greater sensitivity to the dielectric environment, and controllable redirection of EM radiation, closed form expressions are derived for the amplification factor of nanoshell mediated intermolecular energy transfer. Closed form expressions derived in this manuscript can directly be used as formula for; designing SP based biosensors, calculating energy exchange between proteins and excitonic interactions in Quantum Dots (QDs).
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