金纳米二聚体在电磁波谱可见-红外区的热等离子体特性研究

N. Pathak, P. Sarathi
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引用次数: 1

摘要

本文用数值方法研究了金纳米二聚体在局部表面等离子体共振下辐照时产生的热量。采用第一主法进行理论计算,得到了不同参数范围下金纳米二聚体的吸收截面。通过求解依赖于吸收截面和表面等离子体共振波长的稳态传热方程,从温度角度列举了加热机理。这些表面等离子体共振对二聚体之间的距离非常敏感,并且通过管理球体之间的距离从0到6 nm从可见光范围调谐到红外范围。利用边界元法(BEM)对金纳米二聚体在等离子体共振下的归一化电场分布进行了计算,实现了在光学加热应用中起重要作用的局部热点的可视化。该工作为金纳米二聚体的加热机理提供了基本的认识,可以在电磁波谱的可见和近红外区域作为等离子体纳米加热器在多个科学分支中得到应用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Study of thermoplasmonic properties of gold nanodimer in visible -infrared region of electromagnetic spectrum
In the present study, the heat generation in gold nanodimer when irradiated at their localized surface plasmon resonances is investigated numerically. The theoretical calculations are performed employing the first principal approach to obtain the absorption cross-section of gold nanodimer for different parameter ranges. The heating mechanism is enumerated in terms of its temperature by solving the steady-state heat transfer equation which depends on the absorption cross-section and surface plasmon resonance wavelength. These surface plasmon resonances are quite sensitive to the distance between the dimer and have been tuned from visible to IR range by managing the distance between spheres from 0 to 6 nm. The computation of normalized electric field distribution of gold nanodimer under the plasmon resonance has been mapped using boundary element method(BEM) which enables visualization of the local hot spot that plays a significant role in optical heating applications. The work furnishes the basic understanding of the heating mechanism of gold nanodimer which can find application as plasmonic nanoheaters in several branches of science in visible and near-infrared regions of the electromagnetic spectrum.
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CiteScore
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