锆石砂环境安全相关辐射暴露评价

D. D. Lestiani, S. Kurniawati, I. Kusmartini, N. Adventini, Woro Yatu Niken, M. Santoso
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引用次数: 1

摘要

锆石砂是地壳中238 U、232 Th等放射性核素的主要来源之一。在印度尼西亚的邦加勿里洞、婆罗洲和廖内省等几个地方都发现了锆石砂的开采和加工。这些活动有可能对工作区域和周围环境产生一定的放射性暴露。因此,有必要开展锆石砂放射性环境安全暴露评价,以保障工作人员和公众的安全。在这项研究中,使用仪器中子活化分析(INAA)测定和评价了从婆罗洲几个地点收集的锆石砂中铀和钍的浓度。样品在G.A Siwabessy, Serpong反应堆的兔系设施中,以中子通量~ 10 13 n.cm -2 s -1辐照15分钟和2小时,然后用伽马能谱HPGe检测器计数。为了评估分析的准确性,土壤标准物质(RMs)随样品一起分析。标准物质分析结果与鉴定值吻合较好。测量结果表明,铀和钍的浓度随样品来源的不同而变化很大。铀和钍浓度分别为214.8±101.7和209.9±169.0 mg/kg。238 U和232 Th分别为2654±1258 Bq/kg和848±683 Bq/kg。结果表明,年等效剂量平均为2.1±1.04 mSv/年,变化范围为0.4 ~ 5.3 mSv/年。利用INAA对锆石砂进行了表征,结果可靠,可用于评估锆石砂中放射性物质含量水平,与政府对锆石砂放射性暴露的规定有关,以及预防措施,以减少工人和公众的不必要暴露。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Assesment of Environmental Safety Related Radioactivity Exposure In Zircon Sand
Zircon sand is one of major sources that are responsible for naturally occurring radionuclides in the earth’s crust such as 238 U and 232 Th. The mining and processing of zircon sand are found in several places in Indonesia such as in Bangka Belitung, Borneo and Riau. These activities are potential to produce some radioactivity exposure to the occupational area and surrounding environment. Therefore, the assessment of the environmental safety related radioactivity exposure in zircon sands is needed to ensure the safety of the worker and public. In this study, the concentration of uranium and thorium in zircon sands collected from several sites in Borneo were determined and evaluated using instrumental neutron activation analysis (INAA). Samples were irradiated in rabbit system facility of G.A Siwabessy, Serpong reactor with neutron flux ~ 10 13 n.cm -2 .s -1 for 15 minutes and 2 hours, and then counted with HPGe detector of gamma spectrometry. In order to assess the accuracy of the analysis, soil reference materials (RMs) were analyzed together with the samples. The results of reference material analysis showed a good agreement with the certificate value. The measurement results showed that the concentration of uranium and thorium varied widely depending on the sample origin. Uranium and thorium concentrations were 214.8 ± 101.7 and 209.9 ± 169.0 mg/kg, respectively. These values were equivalent to 2654 ± 1258 Bq/kg for 238 U and 848 ± 683 Bq/kg for 232 Th, respectively. The results showed the annual equivalent dose average of 2.1 ± 1.04 mSv/year and varies between 0.4 and 5.3 mSv/year.  The characterization of zircon sands using INAA showed reliable results and could be utilized to assess the level of radioactive materials content in the zircon sands related to government regulation on zircon sand radioactive exposure, as well as the precaution to reduce needless exposure of the workers and public.
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