{"title":"纳米结构二氧化硅气凝胶在近红外波段的大纯折射非线性","authors":"J. Seo, Q. Yang, S. Creekmore, D. Temple","doi":"10.1109/NANO.2002.1032296","DOIUrl":null,"url":null,"abstract":"The nonlinear refraction coefficient of the third-order susceptibility of silica aerogel was estimated to be /spl sim/-1.5/spl times/10/sup -15/ m/sup 2//W (/spl sim/-3.67/spl times/10/sup -9/ esu) by a signal-beam z-scan technique with /spl sim/1 ps Ti:sapphire lasers. The third-order nonlinear refraction coefficient of nanostructure silica aerogel is almost five orders larger than the nonlinear (/spl chi//sup 3/) refraction of bulk material. The large nonlinear refraction originates mainly from the direct excitation to the surface trapped states, and the one-photon resonance process.","PeriodicalId":408575,"journal":{"name":"Proceedings of the 2nd IEEE Conference on Nanotechnology","volume":"110 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2002-11-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"1","resultStr":"{\"title\":\"Large pure refractive nonlinearity of nanostructure silica aerogel at near infrared wavelength\",\"authors\":\"J. Seo, Q. Yang, S. Creekmore, D. Temple\",\"doi\":\"10.1109/NANO.2002.1032296\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The nonlinear refraction coefficient of the third-order susceptibility of silica aerogel was estimated to be /spl sim/-1.5/spl times/10/sup -15/ m/sup 2//W (/spl sim/-3.67/spl times/10/sup -9/ esu) by a signal-beam z-scan technique with /spl sim/1 ps Ti:sapphire lasers. The third-order nonlinear refraction coefficient of nanostructure silica aerogel is almost five orders larger than the nonlinear (/spl chi//sup 3/) refraction of bulk material. The large nonlinear refraction originates mainly from the direct excitation to the surface trapped states, and the one-photon resonance process.\",\"PeriodicalId\":408575,\"journal\":{\"name\":\"Proceedings of the 2nd IEEE Conference on Nanotechnology\",\"volume\":\"110 1\",\"pages\":\"0\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2002-11-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"1\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Proceedings of the 2nd IEEE Conference on Nanotechnology\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1109/NANO.2002.1032296\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Proceedings of the 2nd IEEE Conference on Nanotechnology","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1109/NANO.2002.1032296","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Large pure refractive nonlinearity of nanostructure silica aerogel at near infrared wavelength
The nonlinear refraction coefficient of the third-order susceptibility of silica aerogel was estimated to be /spl sim/-1.5/spl times/10/sup -15/ m/sup 2//W (/spl sim/-3.67/spl times/10/sup -9/ esu) by a signal-beam z-scan technique with /spl sim/1 ps Ti:sapphire lasers. The third-order nonlinear refraction coefficient of nanostructure silica aerogel is almost five orders larger than the nonlinear (/spl chi//sup 3/) refraction of bulk material. The large nonlinear refraction originates mainly from the direct excitation to the surface trapped states, and the one-photon resonance process.
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