PEM燃料电池多孔介质压缩对面内输运现象的影响

IF 5.4 Q2 CHEMISTRY, PHYSICAL
Mehdi Mortazavi , Anthony D. Santamaria , Vedang Chauhan , Jingru Z. Benner , Mahbod Heidari , Ezequiel F. Médici
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引用次数: 24

摘要

采用非原位实验装置研究了质子交换膜燃料电池气体扩散层内液气两相流动。研究了碳纸和碳布在不同压缩率下的质量输运现象。用CCD相机观察了水在GDL平面内的渗透情况,同时测量了其注入压力。同样,研究了初始饱和水的GDL样品平面内的空气渗透。对稳定驱替、毛细指法和粘性指法三种流动形式进行了实验研究。对图像进行分析,得到归一化的湿化面积。研究发现,对于稳定位移和粘性指法流动,GDL压缩直接影响归一化润湿面积,而对于毛细指法流动,GDL压缩对归一化润湿面积没有影响。对于稳定的位移流态,对于碳纸和碳布样品,水渗透压力随着GDL压缩而增加。然而,从毛细指指流动状态中获得的水渗透压力数据并没有显示出任何明显的趋势,作为GDL压缩的函数。本研究结果可用于验证孔隙网络模型等不同方案提出的渗流模型。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Effect of PEM fuel cell porous media compression on in-plane transport phenomena

Liquid-gas two-phase flow in the gas diffusion layer (GDL) of proton exchange membrane fuel cells is investigated using an ex-situ experimental setup. The mass transport phenomena is investigated in carbon paper and carbon cloth GDLs and at different compressions. Water percolation within the plane of the GDL is visualized with a CCD camera while its injection pressure is measured. Similarly, air percolation within the plane of GDL samples which were initially saturated with water is investigated. Experiments are conducted for the three flow regimes of stable displacement, capillary fingering, and viscous fingering. Images are analyzed to obtain the normalized wetted area. It is observed that while the GDL compression directly affects normalized wetted area for stable displacement and viscous fingering flow regimes, it has no impact on this parameter for capillary fingering flow regime. For stable displacement flow regime and for both carbon paper and carbon cloth samples, water percolation pressure increases with GDL compression. However, the water percolation pressure data obtained for capillary fingering flow regime does not suggest any discernible trend as a function of GDL compression. The findings in this study can be used to validate percolation models proposed by different schemes such as pore-network models.

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来源期刊
CiteScore
9.10
自引率
0.00%
发文量
18
审稿时长
64 days
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