Solar-light-induced green conversion of amines into imines by lemon derived heteroatoms-doped GQDs as a green photocatalyst

IF 1.3 4区化学 Q3 CHEMISTRY, MULTIDISCIPLINARY

Main Group Chemistry Pub Date : 2022-12-23 DOI:10.3233/mgc-220094

Satyam Singh, R. Yadav, T. W. Kim, P. Pande, Surabhi Chaubey, Ashutosh Kumar Singh

引用次数: 1

Abstract

Graphene is one of the amazing present encroachments in current research area of science and one of the utmost fascinating materials for relevance in cutting-edge research. Herein, we designed lemon-derived heteroatoms-doped graphene quantum dots (S, N-GQDs) based photocatalyst for the first time. For the integrating reactions of amines in aerobic conditions under solar light by S, N-GQDs photocatalyst exhibit utmost higher photocatalytic activity than simple oxygen-doped graphene quantum dots (O-GQDs) due to slow recombination charges. The mechanisms accountable for the drastically increased photocatalytic activity of S, N-GQDs in solar light responsive integrating reactions of amines in aerobic conditions into the corresponding derivative of imines are also completely scrutinized.

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柠檬衍生杂原子掺杂GQDs作为绿色光催化剂在日光诱导下将胺转化为亚胺

石墨烯是当前科学研究领域中令人惊叹的新进展之一，也是与前沿研究相关的最具吸引力的材料之一。本文首次设计了柠檬衍生的杂原子掺杂石墨烯量子点(S, N-GQDs)光催化剂。由于复合电荷缓慢，N-GQDs光催化剂表现出比单纯掺氧石墨烯量子点(O-GQDs)更高的光催化活性。S, N-GQDs在好氧条件下对太阳光响应的胺与相应亚胺衍生物的整合反应中的光催化活性急剧增加的机制也得到了全面的审查。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Main Group Chemistry 化学-化学综合

CiteScore

2.00

自引率

26.70%

发文量

审稿时长

>12 weeks

期刊介绍： Main Group Chemistry is intended to be a primary resource for all chemistry, engineering, biological, and materials researchers in both academia and in industry with an interest in the elements from the groups 1, 2, 12–18, lanthanides and actinides. The journal is committed to maintaining a high standard for its publications. This will be ensured by a rigorous peer-review process with most articles being reviewed by at least one editorial board member. Additionally, all manuscripts will be proofread and corrected by a dedicated copy editor located at the University of Kentucky.