Analytical Description of Concentration of Radiation Displacement Defects in Oxide Crystals as Function of Electrons or Neutrons Energy

IF 1.5 Q4 MATERIALS SCIENCE, MULTIDISCIPLINARY
P. Potera
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Abstract

Abstract The main purpose of this work is the description of dependence of the concentration of radiation displacements defects (RDD) induced by electrons and neutrons in garnets, perovskites, silicates, germanates, and tungsted bronzes type crystals (Y3Al5O12, Gd3Ga5O12, YAlO3, LiNbO3, Bi4Si3O12, Bi4Ge3O12, Ca0.28Ba0.72Nb2O6) on the energy of particles by analytical function. The dependences were determined on the basis of calculations made using the Monte-Carlo method realized in the Atom Collision Cascade Simulation program. The results of calculations show that the concentrations of RDD reduced to one impinging particle increased initially with the particles energy and they saturates for the electron and neutron energy above 3–36 MeV, depending on crystal, sublattice and kind of irradiation particle. A wide range of energies for which the concentration of RDD is independent of the energy of particles (neutrons, electrons) makes them potential materials for the dosimetry of high-energy particles. The comparison of the concentrations of RDD calculated for different sublattices as well as for the cases of electrons and neutrons is made. In the case of irradiation with electrons, the relative concentration of RDD of the oxygen sublattice strongly depends on the energy of electrons and the crystal and varies in the range of 10–90%. In the case of neutrons, the relative concentration of RDD of the oxygen sublattice does not depend on the neutron energy and is in the range of 66–84% depending on the crystal.
氧化晶体中辐射位移缺陷浓度随电子或中子能量函数的解析描述
摘要本文的主要目的是用解析函数描述石榴石、钙钛矿、硅酸盐、锗酸盐和钨青铜型晶体(Y3Al5O12、Gd3Ga5O12、YAlO3、LiNbO3、Bi4Si3O12、Bi4Ge3O12、Ca0.28Ba0.72Nb2O6)中电子和中子诱导的辐射位移缺陷(RDD)浓度与粒子能量的关系。根据在原子碰撞级联模拟程序中实现的蒙特卡罗方法进行的计算确定了依赖关系。计算结果表明,随着粒子能量的增加,RDD的浓度开始增加,在电子和中子能量高于3 - 36mev时,RDD的浓度达到饱和,这取决于晶体、亚晶格和辐照粒子的种类。RDD的浓度与粒子(中子、电子)的能量无关的能量范围很广,这使它们成为高能粒子剂量测定的潜在材料。比较了不同亚晶格的RDD浓度,以及电子和中子的RDD浓度。在电子辐照的情况下,氧亚晶格RDD的相对浓度与电子和晶体的能量密切相关,在10-90%的范围内变化。在中子的情况下,氧亚晶格RDD的相对浓度不依赖于中子能量,根据晶体的不同,RDD的相对浓度在66-84%之间。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Advances in Materials Science
Advances in Materials Science MATERIALS SCIENCE, MULTIDISCIPLINARY-
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