Investigation of Temperature Dependency on the Propulsion of Disk-like Nanoswimmers

Liangxing Hu , Nan Wang , Jianmin Miao , Gerhard Grüber
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引用次数: 7

Abstract

Flight vehicles can soar around Earth via ejecting the combusted gases in the space and bio-molecular motor proteins possess the ability to walk along the tracts through hydrolyzing adenosine triphosphate (ATP) in cells. Inspired by flight vehicles and naturally occurring bio-molecular protein motors, miniaturized disk-like nanoswimmers are proposed, which are composed of three different metals: gold (Au), nickel (Ni), and platinum (Pt). The proposed nanoswimmers are fabricated via a layer-by-layer deposition method base on nano-electro-mechanical systems (NEMS) technology, whereby Pt functions as the chemical catalyst for the decomposition of hydrogen peroxide (H2O2) to produce oxygen (O2) bubbles detaching from its surface, which in turn generate recoil force to thrust nanoswimmers propelling forward. Herein, bubble propulsion mechanism originating from momentum change of a Au-Ni-Pt nanoswimmer-O2 bubble integral system is proposed to investigate the propulsion of nanoswimmers. Experiments are mainly focused on characterizing the propulsion of nanoswimmers in diluted H2O2 by changing the temperature of the solution. Results show that Au-Ni-Pt nanoswimmers are able to propel forward while the generated O2 bubbles are detached from the Pt-surface. The speeds of nanoswimmers are increased with the increment of temperature varying from 7 °C to 57 °C. It is concluded that the propulsion of nanoswimmers is temperature-dependent.

盘状纳米游泳器推进的温度依赖性研究
飞行器可以通过在太空中喷射燃烧气体在地球周围翱翔,生物分子马达蛋白具有通过水解细胞中的三磷酸腺苷(ATP)沿着束行走的能力。受飞行器和自然存在的生物分子蛋白质马达的启发,提出了小型化的圆盘状纳米游泳器,它由三种不同的金属组成:金(Au),镍(Ni)和铂(Pt)。所提出的纳米游泳体是通过基于纳米机电系统(NEMS)技术的逐层沉积方法制造的,其中Pt作为过氧化氢(H2O2)分解的化学催化剂,产生从其表面分离的氧(O2)气泡,这些气泡反过来产生后坐力,推动纳米游泳体向前推进。本文提出了由Au-Ni-Pt纳米游泳分子- o2气泡积分体系动量变化引起的气泡推进机制,以研究纳米游泳分子的推进作用。实验主要集中在通过改变溶液温度来表征纳米游泳者在稀释H2O2中的推进特性。结果表明,Au-Ni-Pt纳米游泳者能够在产生的O2气泡与pt表面分离的情况下向前推进。在7 ~ 57℃温度范围内,纳米游泳者的速度随温度的升高而增加。结果表明,纳米游泳者的推进力与温度有关。
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