Chlorine-doped perovskite materials for highly efficient perovskite solar cell design offering an efficiency of nearly 29%

IF 8 2区材料科学 Q1 ENERGY & FUELS

Progress in Photovoltaics Pub Date : 2023-08-10 DOI:10.1002/pip.3732

Sagar Bhattarai, Rahul Pandey, Jaya Madan, Mohd Zahid Ansari, M. Khalid Hossain, Mongi Amami, Shaik Hasane Ahammad, Ahmed Nabih Zaki Rashed

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引用次数: 3

Abstract

The new form of renewable energy attracts enormous attention from researchers for its immense importance and impact on our daily life. A fossil energy is a non-renewable source that will end shortly because of its immense use in houses and industries. Among the renewable sources, solar cells based on perovskite (PVK) materials exponentially increase their efficiency from 3.8% to 25.8% rapidly in a diminutive period of time. In the present study, doped and undoped PVK layers (MAPbI₃, MAPb[I_1-xCl_x]₃) are considered and optimized for solar cell application by using the SCAPS-1D device simulator. A detailed investigation is done in terms of PVK absorber layer (PAL) thickness variation with different electron and hole transport layers, temperature, and bulk defect density to optimize the device performance. The MAPb(I_1-xCl_x)₃-based device delivered the highest conversion efficiency of ~29% with J_SC of 25.59 mA/cm², V_OC of 1.348 Volt, and an FF of about 83.68%. Results reported in this work may pave the way for the development of advanced high-efficiency PVK solar cells.

Abstract Image

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掺氯过氧化物材料用于高效过氧化物太阳能电池设计，效率接近 29

新形式的可再生能源因其对我们日常生活的巨大重要性和影响而备受研究人员的关注。化石能源是一种不可再生能源，由于其在住宅和工业中的大量使用，这种能源很快就会消失。在可再生能源中，基于包晶体（PVK）材料的太阳能电池能在很短的时间内将效率从 3.8% 迅速提高到 25.8%。本研究使用 SCAPS-1D 设备模拟器，考虑并优化了掺杂和未掺杂 PVK 层（MAPbI3、MAPb[I1-xClx]3）在太阳能电池中的应用。详细研究了 PVK 吸收层（PAL）厚度随不同电子和空穴传输层、温度和体缺陷密度的变化，以优化器件性能。基于 MAPb（I1-xClx）3 的器件转换效率最高，达到约 29%，JSC 为 25.59 mA/cm2，VOC 为 1.348 Volt，FF 约为 83.68%。这项工作所报告的结果可为开发先进的高效 PVK 太阳能电池铺平道路。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Progress in Photovoltaics 工程技术-能源与燃料

CiteScore

18.10

自引率

7.50%

发文量

130

审稿时长

5.4 months

期刊介绍： Progress in Photovoltaics offers a prestigious forum for reporting advances in this rapidly developing technology, aiming to reach all interested professionals, researchers and energy policy-makers. The key criterion is that all papers submitted should report substantial “progress” in photovoltaics. Papers are encouraged that report substantial “progress” such as gains in independently certified solar cell efficiency, eligible for a new entry in the journal''s widely referenced Solar Cell Efficiency Tables. Examples of papers that will not be considered for publication are those that report development in materials without relation to data on cell performance, routine analysis, characterisation or modelling of cells or processing sequences, routine reports of system performance, improvements in electronic hardware design, or country programs, although invited papers may occasionally be solicited in these areas to capture accumulated “progress”.