Catalytic membrane reactors for carbon peaking and carbon neutrality

Jiuxuan Zhang , Bo Liu , Lili Cai , Yanhong Li , Yan Zhang , Mengke Liu , Lujian Jia , Senqing Fan , Linfeng Lei , Minghui Zhu , Xuefeng Zhu , Xuebin Ke , Aisheng Huang , Heqing Jiang , Rizhi Chen
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Abstract

Catalytic membrane reactors have the advantages of allowing the selective removal of products, avoiding the separation procedure of powder catalysts from the reaction mixture, intensifying the diffusion of reactants in the catalytic region, and integrating different reactions in one unit. Catalytic membrane reactors have been widely applied in the fields related to carbon peaking and carbon neutrality, including the capture and utilization of carbon dioxide, hydrogen production, and hydrogenation reaction. This review summarizes the design and fabrication of catalytic membrane reactors, with the focus on the capture and efficient utilization of carbon dioxide, hydrogen production and efficient liquid-phase hydrogenation. The design of membrane materials, catalyst materials and catalytic membranes, and the operation of catalytic membrane reactors are discussed respectively. Finally, the perspectives and future challenges of catalytic membrane reactors for carbon peaking and carbon neutrality are forecasted.

Abstract Image

用于碳达峰和碳中和的催化膜反应器
催化膜反应器的优点是可以选择性地去除产物,避免了粉末催化剂从反应混合物中分离的过程,增强了反应物在催化区的扩散,并将不同的反应整合在一个单元中。催化膜反应器已广泛应用于碳达峰和碳中和相关领域,包括二氧化碳的捕获和利用、制氢和加氢反应。本文综述了催化膜反应器的设计和制造,重点介绍了二氧化碳的捕获和高效利用、氢气生产和高效液相加氢。分别讨论了膜材料、催化剂材料和催化膜的设计以及催化膜反应器的操作。最后,展望了催化膜反应器在碳达峰和碳中和方面的前景和未来挑战。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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