Influence of different CO2 phase states on fluid flow pathways in coal: insights from image reconstruction and fractal study

IF 3.7 2区 工程技术 Q3 ENGINEERING, ENVIRONMENTAL
Peng Luo, Zhenyu Zhang, Lei Zhang, Xiaoqian Liu, Xiaobo Liu
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Abstract

The CO2 phase state changes during the long-term interaction with coal seams. A proper understanding of the influence of different CO2 phase states in water-bearing coal seams is of great significance in evaluating the leakage risk during CO2 sequestration. The evolution of fluid flow pathways in water-bearing coal subjected to the treatment of different CO2 phase states was investigated by using X-ray computed tomography (CT) technology, fractal dimension, and three-dimensional (3D) pore-scale flow modeling. The results show that the supercritical CO2 (ScCO2) treatment reduced the coal heterogeneity by 12.69% and increased the absolute permeability by 58.75%. Conversely, only 0.71% of coal heterogeneity reduction occurred after subcritical CO2 (SubCO2) treatment, increasing the absolute permeability by 24.91%. The reduction in the tortuosity fractal dimension after ScCO2 treatment was 2.69% larger than that of SubCO2 treatment, indicating that ScCO2 treatment was more favorable for improving the transport capacity of flow pathways. The pressure field distributions in the pore network model (PNM) were determined by coal heterogeneity and influenced by the number of flow pathways. The effect of ScCO2 treatment on the size, quantity, and location of preferential flow pathways in coal is more significant than that of SubCO2 treatment. Moreover, the proportion of preferential flow pathways in ScCO2-treated coal was less than 50%, much lower than that of the throats in PNMs. In contrast, the proportion of preferential flow pathways in SubCO2-treated coal was approximately 30% higher than that in ScCO2-treated coal. The distribution of preferential flow pathways also indicated that not all pores with larger radii participated in preferential flow. Furthermore, more than 50% of the pathways in the ScCO2-treated coal did not contribute to fluid flow, and could affect the stability of the coal seam.

Abstract Image

不同CO2相态对煤中流体流动路径的影响——来自图像重建和分形研究的启示
在与煤层的长期相互作用过程中,CO2的相态发生了变化。正确认识含水煤层中不同CO2相态的影响对评价CO2封存过程的泄漏风险具有重要意义。采用x射线计算机断层扫描(CT)技术、分形维数和三维(3D)孔隙尺度流动模型研究了不同CO2相态处理下含水煤流体流动路径的演化。结果表明:超临界CO2处理使煤的非均质性降低了12.69%,绝对渗透率提高了58.75%;相反,亚临界CO2 (SubCO2)处理后,煤的非均质性仅降低0.71%,绝对渗透率提高24.91%。ScCO2处理后的弯曲度分形维数降幅比SubCO2处理大2.69%,表明ScCO2处理更有利于提高流动通道的输送能力。孔隙网络模型(PNM)中的压力场分布由煤的非均质性决定,并受流道数的影响。ScCO2处理对煤中优先流动通道的大小、数量和位置的影响比SubCO2处理更显著。此外,scco2处理煤中优先流动通道的比例小于50%,远低于pmms中喉道的比例。相比之下,subco2处理煤中优先流动路径的比例比scco2处理煤高约30%。优先流动通道的分布也表明,并非所有半径较大的孔隙都参与了优先流动。此外,scco2处理煤中超过50%的路径不利于流体流动,可能影响煤层的稳定性。
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来源期刊
Bulletin of Engineering Geology and the Environment
Bulletin of Engineering Geology and the Environment 工程技术-地球科学综合
CiteScore
7.10
自引率
11.90%
发文量
445
审稿时长
4.1 months
期刊介绍: Engineering geology is defined in the statutes of the IAEG as the science devoted to the investigation, study and solution of engineering and environmental problems which may arise as the result of the interaction between geology and the works or activities of man, as well as of the prediction of and development of measures for the prevention or remediation of geological hazards. Engineering geology embraces: • the applications/implications of the geomorphology, structural geology, and hydrogeological conditions of geological formations; • the characterisation of the mineralogical, physico-geomechanical, chemical and hydraulic properties of all earth materials involved in construction, resource recovery and environmental change; • the assessment of the mechanical and hydrological behaviour of soil and rock masses; • the prediction of changes to the above properties with time; • the determination of the parameters to be considered in the stability analysis of engineering works and earth masses.
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