{"title":"Photoinduced self-assembly of nanocrystals inside Al2O3-Lu2O3 glass","authors":"T. Okuno, Y. Shimotsuma, M. Shimizu, K. Miura","doi":"10.3389/aot.2023.1237663","DOIUrl":null,"url":null,"abstract":"The femtosecond laser direct writing technique can allow spatially selective crystallization with suppression of thermal conduction effects. In the case of Al2O3-R2O3 (R = Y, Dy) glass, the polarization-dependent periodic nanostructure with crystallization is self-assembled, however, the formation mechanism of self-assembled nanocrystals in glass remains to be clarified. We focused on Al2O3-Lu2O3 glass prepared by a containerless laser melting method and demonstrated the formation of a nanograting with crystallization by femtosecond laser irradiation. Polarized luminescence measurements of the crystallized region by the pulse bursts with a controllable number of pulses reveal that luminescence anisotropy increased at more than 50 pulses in a burst, suggesting the formation of the nanograting. We have also followed the time variation of birefringence by polarized light imaging to evaluate the time scale for the formation of nanogratings with crystallization.","PeriodicalId":46010,"journal":{"name":"Advanced Optical Technologies","volume":null,"pages":null},"PeriodicalIF":2.3000,"publicationDate":"2023-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Optical Technologies","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.3389/aot.2023.1237663","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"OPTICS","Score":null,"Total":0}
引用次数: 0
Abstract
The femtosecond laser direct writing technique can allow spatially selective crystallization with suppression of thermal conduction effects. In the case of Al2O3-R2O3 (R = Y, Dy) glass, the polarization-dependent periodic nanostructure with crystallization is self-assembled, however, the formation mechanism of self-assembled nanocrystals in glass remains to be clarified. We focused on Al2O3-Lu2O3 glass prepared by a containerless laser melting method and demonstrated the formation of a nanograting with crystallization by femtosecond laser irradiation. Polarized luminescence measurements of the crystallized region by the pulse bursts with a controllable number of pulses reveal that luminescence anisotropy increased at more than 50 pulses in a burst, suggesting the formation of the nanograting. We have also followed the time variation of birefringence by polarized light imaging to evaluate the time scale for the formation of nanogratings with crystallization.
期刊介绍:
Advanced Optical Technologies is a strictly peer-reviewed scientific journal. The major aim of Advanced Optical Technologies is to publish recent progress in the fields of optical design, optical engineering, and optical manufacturing. Advanced Optical Technologies has a main focus on applied research and addresses scientists as well as experts in industrial research and development. Advanced Optical Technologies partners with the European Optical Society (EOS). All its 4.500+ members have free online access to the journal through their EOS member account. Topics: Optical design, Lithography, Opto-mechanical engineering, Illumination and lighting technology, Precision fabrication, Image sensor devices, Optical materials (polymer based, inorganic, crystalline/amorphous), Optical instruments in life science (biology, medicine, laboratories), Optical metrology, Optics in aerospace/defense, Simulation, interdisciplinary, Optics for astronomy, Standards, Consumer optics, Optical coatings.