Advances in carbon nitride supported single-atom photocatalysts for hydrogen evolution

IF 8 2区 工程技术 Q1 BIOTECHNOLOGY & APPLIED MICROBIOLOGY
Fanpeng Meng , Zhihao Tian , Wenjie Tian , Huayang Zhang
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引用次数: 3

Abstract

Owing to their distinct collaboration nature, high atom usage, and high catalytic performance, single-atom catalysts have become most dynamically studied in various catalytic reactions. Graphitic carbon nitride (g-C3N4), as one of the most promising two-dimensional supports for stable immobilization of single-atom metals, has received extensive investigations. In this review, the recent developments of g-C3N4-supported single-atom photocatalysts for hydrogen evolution are summarized, with the metal-support interactions and structure regulations for stable and efficient catalysis being highlighted. Finally, the difficulties and potentials for future development of g-C3N4-supported single-atom materials in photocatalytic hydrogen evolution are proposed.

Abstract Image

氮化碳负载单原子析氢光催化剂的研究进展
单原子催化剂由于其独特的协同性质、高原子利用率和高催化性能,在各种催化反应中得到了最动态的研究。石墨氮化碳(g-C3N4)作为一种最有前途的稳定固定单原子金属的二维载体,受到了广泛的研究。本文综述了近年来g- c3n4负载单原子析氢催化剂的研究进展,重点介绍了g- c3n4负载单原子析氢催化剂的金属-载体相互作用和结构规律。最后,提出了g- c3n4负载单原子材料光催化析氢的难点和未来发展潜力。
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来源期刊
Current Opinion in Chemical Engineering
Current Opinion in Chemical Engineering BIOTECHNOLOGY & APPLIED MICROBIOLOGYENGINE-ENGINEERING, CHEMICAL
CiteScore
12.80
自引率
3.00%
发文量
114
期刊介绍: Current Opinion in Chemical Engineering is devoted to bringing forth short and focused review articles written by experts on current advances in different areas of chemical engineering. Only invited review articles will be published. The goals of each review article in Current Opinion in Chemical Engineering are: 1. To acquaint the reader/researcher with the most important recent papers in the given topic. 2. To provide the reader with the views/opinions of the expert in each topic. The reviews are short (about 2500 words or 5-10 printed pages with figures) and serve as an invaluable source of information for researchers, teachers, professionals and students. The reviews also aim to stimulate exchange of ideas among experts. Themed sections: Each review will focus on particular aspects of one of the following themed sections of chemical engineering: 1. Nanotechnology 2. Energy and environmental engineering 3. Biotechnology and bioprocess engineering 4. Biological engineering (covering tissue engineering, regenerative medicine, drug delivery) 5. Separation engineering (covering membrane technologies, adsorbents, desalination, distillation etc.) 6. Materials engineering (covering biomaterials, inorganic especially ceramic materials, nanostructured materials). 7. Process systems engineering 8. Reaction engineering and catalysis.
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