How Temperature Measurement Impacts Pressure Drop and Heat Transport in Slender Fixed Beds of Raschig Rings

IF 4.3 Q2 ENGINEERING, CHEMICAL
Martin Kutscherauer, Philipp Reinold, Sebastian Böcklein, Gerhard Mestl, Thomas Turek and Gregor D. Wehinger*, 
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引用次数: 1

Abstract

The axial temperature profile of a packed bed is often measured by thermocouples placed either directly in the bed or inside a thermowell centered in the reactor tube. Quantifying the impact of the thermocouple well on fluid flow, heat transport, and consequently on the measured temperatures is still an unresolved challenge for lab-scale reactors but especially, and even more so for multitubular reactors in industry. Particle-resolved computational fluid dynamics (PRCFD) simulations are a suitable approach to investigate the changes in transport phenomena exerted by inserting thermocouple wells into packed beds because they take into account the local packed bed structures. In this study, PRCFD simulations are performed based on design of simulation experiments (DoSE). The effect of the thermowell diameter and its thermal conductivity on the deviations between packed beds with and without thermowells is statistically quantified for characteristic integral quantities like pressure drop and tube wall-bed Nusselt number. The axial temperature profiles inside the thermowells can be computed efficiently with reasonably accuracy applying the Nusselt number correction as derived in this study from the DoSE in a one-dimensional pseudo-homogeneous energy balance.

Abstract Image

温度测量对细长拉希环固定床压降和热传递的影响
填充床的轴向温度分布通常是通过直接放置在床上或放置在反应器管中心的热电偶来测量的。量化热电偶对流体流动、热传递以及测量温度的影响对于实验室规模的反应器来说仍然是一个未解决的挑战,特别是对于工业上的多管反应器来说更是如此。粒子解析计算流体动力学(PRCFD)模拟是研究热电偶井插入充填床后输运现象变化的一种合适方法,因为它考虑了充填床的局部结构。在本研究中,基于模拟实验设计(DoSE)进行了PRCFD模拟。利用压降和管壁床努塞尔数等特征积分,统计量化了热电偶直径及其导热系数对有热电偶和无热电偶填料床间偏差的影响。在一维拟均匀能量平衡中,应用本文导出的努塞尔数校正,可以有效地计算热电偶井内的轴向温度分布,并具有合理的精度。
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来源期刊
ACS Engineering Au
ACS Engineering Au 化学工程技术-
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期刊介绍: )ACS Engineering Au is an open access journal that reports significant advances in chemical engineering applied chemistry and energy covering fundamentals processes and products. The journal's broad scope includes experimental theoretical mathematical computational chemical and physical research from academic and industrial settings. Short letters comprehensive articles reviews and perspectives are welcome on topics that include:Fundamental research in such areas as thermodynamics transport phenomena (flow mixing mass & heat transfer) chemical reaction kinetics and engineering catalysis separations interfacial phenomena and materialsProcess design development and intensification (e.g. process technologies for chemicals and materials synthesis and design methods process intensification multiphase reactors scale-up systems analysis process control data correlation schemes modeling machine learning Artificial Intelligence)Product research and development involving chemical and engineering aspects (e.g. catalysts plastics elastomers fibers adhesives coatings paper membranes lubricants ceramics aerosols fluidic devices intensified process equipment)Energy and fuels (e.g. pre-treatment processing and utilization of renewable energy resources; processing and utilization of fuels; properties and structure or molecular composition of both raw fuels and refined products; fuel cells hydrogen batteries; photochemical fuel and energy production; decarbonization; electrification; microwave; cavitation)Measurement techniques computational models and data on thermo-physical thermodynamic and transport properties of materials and phase equilibrium behaviorNew methods models and tools (e.g. real-time data analytics multi-scale models physics informed machine learning models machine learning enhanced physics-based models soft sensors high-performance computing)
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