3D-printed amperometric sensor for the detection of ethanol in saliva

IF 2.7 3区 化学 Q2 CHEMISTRY, ANALYTICAL
Theodora Wrobel von Zuben, Cristiane Kalinke, Bruno Campos Janegitz, Airton Gonçalves Salles Jr., Juliano Alves Bonacin
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引用次数: 0

Abstract

In this work, we report a non-enzymatic and metal-free ethanol sensor based on 3D PLA-graphene electrodes. We evaluated the optimal activation treatment for PLA-graphene to achieve a sensor for monitoring ethanol levels in saliva samples, following the legal limits for drivers in various countries. The analytical performance of the sensor was determined through amperometric measurements, demonstrating a linear detection ranging supporting electrolyte (0.990–19.3 mmol L−1) and artificial saliva sample (0.990–17.4 mmol L−1), with respective limits of detection of 0.135 and 0.239 mmol L−1. The 3D-printed sensor exhibited excellent repeatability and reproducibility. This method was effectively employed for ethanol detection, highlighting its potential as an alternative approach for assessing ethanol levels in drivers while considering diverse legal regulations across different countries.

Abstract Image

用于检测唾液中乙醇的3D打印电流传感器
在这项工作中,我们报道了一种基于3D PLA石墨烯电极的非酶和无金属乙醇传感器。我们评估了PLA石墨烯的最佳活化处理,以实现监测唾液样本中乙醇水平的传感器,遵循各国对驾驶员的法律限制。传感器的分析性能是通过安培测量确定的,证明了支持电解质(0.990−19.3 mmol L-1)和人工唾液样品(0.990–17.4 mmol L‐1)的线性检测范围,检测限分别为0.135和0.239 mmol L−1。3D打印传感器表现出优异的可重复性和再现性。该方法被有效地用于乙醇检测,突出了其作为评估驾驶员乙醇水平的替代方法的潜力,同时考虑到不同国家的不同法律法规。
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来源期刊
Electroanalysis
Electroanalysis 化学-电化学
CiteScore
6.00
自引率
3.30%
发文量
222
审稿时长
2.4 months
期刊介绍: Electroanalysis is an international, peer-reviewed journal covering all branches of electroanalytical chemistry, including both fundamental and application papers as well as reviews dealing with new electrochemical sensors and biosensors, nanobioelectronics devices, analytical voltammetry, potentiometry, new electrochemical detection schemes based on novel nanomaterials, fuel cells and biofuel cells, and important practical applications. Serving as a vital communication link between the research labs and the field, Electroanalysis helps you to quickly adapt the latest innovations into practical clinical, environmental, food analysis, industrial and energy-related applications. Electroanalysis provides the most comprehensive coverage of the field and is the number one source for information on electroanalytical chemistry, electrochemical sensors and biosensors and fuel/biofuel cells.
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