Degradation of organic pollutants from water by biochar-assisted advanced oxidation processes: Mechanisms and applications

IF 12.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Tao Jiang , Bing Wang , Bin Gao , Ning Cheng , Qianwei Feng , Miao Chen , Shengsen Wang
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引用次数: 38

Abstract

Biochar has shown large potential in environmental remediation because of its low cost, large specific surface area, porosity, and high conductivity. Biochar-assisted advanced oxidation processes (BC-AOPs) have recently attracted increasing attention to the remediation of organic pollutants from water. However, the effects of biochar properties on catalytic performance need to be further explored. There are still controversial and knowledge gaps in the reaction mechanisms of BC-AOPs, and regeneration methods of biochar catalysts are lacking. Therefore, it is necessary to systematically review the latest research progress of BC-AOPs in the treatment of organic pollutants in water. In this review, first of all, the effects of biochar properties on catalytic activity are summarized. The biochar properties can be optimized by changing the feedstocks, preparation conditions, and modification methods. Secondly, the catalytic active sites and degradation mechanisms are explored in different BC-AOPs. Different influencing factors on the degradation process are analyzed. Then, the applications of BC-AOPs in environmental remediation and regeneration methods of different biochar catalysts are summarized. Finally, the development prospects and challenges of biochar catalysts in environmental remediation are put forward, and some suggestions for future development are proposed.

生物炭辅助高级氧化法降解水中有机污染物:机理与应用
生物炭具有成本低、比表面积大、孔隙率高、电导率高等特点,在环境修复中具有很大的应用潜力。近年来,生物炭辅助高级氧化法(BC-AOPs)在水中有机污染物的修复中受到越来越多的关注。然而,生物炭性质对催化性能的影响还有待进一步研究。BC-AOPs的反应机理仍存在争议和知识空白,生物炭催化剂的再生方法也缺乏。因此,有必要对BC-AOPs在处理水中有机污染物方面的最新研究进展进行系统综述。本文首先综述了生物炭性质对催化活性的影响。通过改变原料、制备条件和改性方法,可以优化生物炭的性能。其次,探讨了不同BC-AOPs的催化活性位点和降解机理。分析了不同因素对降解过程的影响。总结了BC-AOPs在不同生物炭催化剂的环境修复和再生方法中的应用。最后,提出了生物炭催化剂在环境修复中的发展前景和面临的挑战,并对未来的发展提出了建议。
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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