Flexible and high-sensitivity sensor based on Ti3C2–MoS2 MXene composite for the detection of toxic gases

IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Van Thuan Le , Yasser Vasseghian , Van Dat Doan , Thi Thu Trang Nguyen , Thu-Thao Thi Vo , Ha Huu Do , Khanh B. Vu , Quang Hieu Vu , Tran Dai Lam , Vy Anh Tran
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引用次数: 46

Abstract

It is vital to have high sensitivity in gas sensors to allow the exact detection of dangerous gases in the air and at room temperature. In this study, we used 2D MXenes and MoS2 materials to create a Ti3C2–MoS2 composite with high metallic conductivity and a wholly functionalized surface for a significant signal. At room temperature, the Ti3C2–MoS2 composite demonstrated clear signals, cyclic response curves to NO2 gas, and gas concentration-dependent. The sensitivities of the standard Ti3C2–MoS2 (TM_2) composite (20 wt% MoS2) rose dramatically to 35.8%, 63.4%, and 72.5% when increasing NO2 concentrations to 10 ppm, 50 ppm, and 100 ppm, respectively. In addition, the composite showed reaction signals to additional hazardous gases, such as ammonia and methane. Our findings suggest that highly functionalized metallic sensing channels could be used to construct multigas-detecting sensors that are very sensitive in air and at room temperature.

Abstract Image

基于Ti3C2-MoS2 MXene复合材料的柔性高灵敏度传感器,用于有毒气体的检测
至关重要的是,气体传感器具有高灵敏度,以便在空气和室温下精确检测危险气体。在这项研究中,我们使用二维MXenes和MoS2材料创建了具有高金属导电性和完全功能化表面的Ti3C2-MoS2复合材料,用于显著信号。在室温下,Ti3C2-MoS2复合材料表现出清晰的信号,对NO2气体的循环响应曲线,且气体浓度依赖。当NO2浓度增加到10 ppm、50 ppm和100 ppm时,标准Ti3C2-MoS2 (TM_2)复合材料(20 wt% MoS2)的灵敏度分别急剧上升到35.8%、63.4%和72.5%。此外,该复合材料对氨和甲烷等其他有害气体也显示出反应信号。我们的研究结果表明,高度功能化的金属传感通道可用于构建在空气和室温下非常敏感的多气体检测传感器。
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来源期刊
Chemosphere
Chemosphere 环境科学-环境科学
CiteScore
15.80
自引率
8.00%
发文量
4975
审稿时长
3.4 months
期刊介绍: Chemosphere, being an international multidisciplinary journal, is dedicated to publishing original communications and review articles on chemicals in the environment. The scope covers a wide range of topics, including the identification, quantification, behavior, fate, toxicology, treatment, and remediation of chemicals in the bio-, hydro-, litho-, and atmosphere, ensuring the broad dissemination of research in this field.
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