A review of hydrogen/rock/brine interaction: Implications for Hydrogen Geo-storage

IF 32 1区 工程技术 Q1 ENERGY & FUELS
Masoud Aslannezhad , Muhammad Ali , Azim Kalantariasl , Mohammad Sayyafzadeh , Zhenjiang You , Stefan Iglauer , Alireza Keshavarz
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引用次数: 46

Abstract

Hydrogen (H2) is currently considered a clean fuel to decrease anthropogenic greenhouse gas emissions and will play a vital role in climate change mitigation. Nevertheless, one of the primary challenges of achieving a complete H2 economy is the large-scale storage of H2, which is unsafe on the surface because H2 is highly compressible, volatile, and flammable. Hydrogen storage in geological formations could be a potential solution to this problem because of the abundance of such formations and their high storage capacities. Wettability plays a critical role in the displacement of formation water and determines the containment safety, storage capacity, and amount of trapped H2 (or recovery factor). However, no comprehensive review article has been published explaining H2 wettability in geological conditions. Therefore, this review focuses on the influence of various parameters, such as salinity, temperature, pressure, surface roughness, and formation type, on wettability and, consequently, H2 storage. Significant gaps exist in the literature on understanding the effect of organic material on H2 storage capacity. Thus, this review summarizes recent advances in rock/H2/brine systems containing organic material in various geological reservoirs. The paper also presents influential parameters affecting H2 storage capacity and containment safety, including liquid–gas interfacial tension, rock–fluid interfacial tension, and adsorption. The paper aims to provide the scientific community with an expert opinion to understand the challenges of H2 storage and identify storage solutions. In addition, the essential differences between underground H2 storage (UHS), natural gas storage, and carbon dioxide geological storage are discussed, and the direction of future research is presented. Therefore, this review promotes thorough knowledge of UHS, provides guidance on operating large-scale UHS projects, encourages climate engineers to focus more on UHS research, and provides an overview of advanced technology. This review also inspires researchers in the field of climate change to give more credit to UHS studies.

氢/岩/盐水相互作用研究进展:对储氢的启示
氢(H2)目前被认为是减少人为温室气体排放的清洁燃料,将在减缓气候变化方面发挥至关重要的作用。然而,实现完全氢气经济性的主要挑战之一是氢气的大规模储存,这在地面上是不安全的,因为氢气具有高度可压缩性、挥发性和可燃性。在地质构造中储氢可能是解决这一问题的一个潜在解决方案,因为这些构造丰富且储氢能力高。润湿性在地层水的置换中起着至关重要的作用,并决定了储层的安全性、储层容量和捕获H2的数量(或采收率)。然而,目前还没有全面的综述文章来解释地质条件下的H2润湿性。因此,本文将重点介绍各种参数(如盐度、温度、压力、表面粗糙度和地层类型)对润湿性的影响,从而影响H2的储存。在了解有机材料对储氢容量的影响方面,文献中存在明显的空白。因此,本文综述了不同地质储层含有机质岩石/H2/盐水体系研究的最新进展。分析了影响储氢容量和安全壳安全性的参数,包括气液界面张力、岩液界面张力和吸附。本文旨在为科学界提供专家意见,以了解H2存储的挑战并确定存储解决方案。讨论了地下储氢与天然气储氢、二氧化碳地质储氢的本质区别,并提出了今后的研究方向。因此,本综述促进了对UHS的全面了解,为大型UHS项目的运营提供了指导,鼓励气候工程师更多地关注UHS研究,并提供了先进技术的概述。这篇综述也激励了气候变化领域的研究人员更多地信任大学保健处的研究。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Progress in Energy and Combustion Science
Progress in Energy and Combustion Science 工程技术-工程:化工
CiteScore
59.30
自引率
0.70%
发文量
44
审稿时长
3 months
期刊介绍: Progress in Energy and Combustion Science (PECS) publishes review articles covering all aspects of energy and combustion science. These articles offer a comprehensive, in-depth overview, evaluation, and discussion of specific topics. Given the importance of climate change and energy conservation, efficient combustion of fossil fuels and the development of sustainable energy systems are emphasized. Environmental protection requires limiting pollutants, including greenhouse gases, emitted from combustion and other energy-intensive systems. Additionally, combustion plays a vital role in process technology and materials science. PECS features articles authored by internationally recognized experts in combustion, flames, fuel science and technology, and sustainable energy solutions. Each volume includes specially commissioned review articles providing orderly and concise surveys and scientific discussions on various aspects of combustion and energy. While not overly lengthy, these articles allow authors to thoroughly and comprehensively explore their subjects. They serve as valuable resources for researchers seeking knowledge beyond their own fields and for students and engineers in government and industrial research seeking comprehensive reviews and practical solutions.
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