Unlocking Thermoelectric Performance in Cu2SnSe3 Through Controlled Structural Ordering

IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Arthur Wieder,Petr Levinský,Gwladys Steciuk,Pierric Lemoine,Erik Elkaim,Jaafar Ghanbaja,Sylvie Migot,Christine Clément,Ghouti Medjahdi,Lionel Aranda,Bernard Malaman,Gérard Le Caër,Gaëlle Delaizir,Ilayda Terzi,Bertrand Lenoir,Soufiane El Oualid,Christophe Candolfi
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引用次数: 0

Abstract

The polymorphism of the tetrahedrally-bonded semiconductor Cu2SnSe3 can be precisely controlled via post-synthesis annealing. This experimental parameter dictates nanoscale structural disorder, modulating the charge-carrier mobility and thermoelectric efficiency. Our findings establish disorder engineering in diamond-like semiconductors as a powerful strategy to tailor and optimize their functional properties.

Abstract Image

通过控制结构排序解锁Cu2SnSe3的热电性能
通过合成后退火可以精确控制四面体键合半导体Cu2SnSe3的多态性。这个实验参数决定了纳米级结构的无序性,调节了载流子迁移率和热电效率。我们的研究结果建立了类金刚石半导体的无序工程作为定制和优化其功能特性的有力策略。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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