Programmable Organic Light‐Emitting Transistors Enabled by Floating‐Gate Charge Storage

IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jiatong Liu, Zeyi Yan, Pusen Zhang, Xiwei Zheng, Xiteng Li, Zhouying Wu, Jun Han, Meili Xu, Hong Meng
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Abstract

Display technologies for high‐resolution smartphones, wearable screens and near‐eye VR/AR microdisplays increasingly require compact pixel architectures with high aperture ratios. Organic light‐emitting transistors (OLETs) improve functional integration by combining transistor switching and electroluminescence within a single device. However, conventional OLETs still define emission states through instantaneous electrical bias, leaving state storage separated from light emission. The absence of memory‐emission co‐location limits intrinsic state programmability in OLET‐based pixel devices. Here, we report programmable organic light‐emitting transistors (P‐OLETs) based on a floating‐gate architecture, in which charge storage enables reversible charge trapping and release, producing programmable switching behavior and tunable electroluminescence. The stored charge modulates channel transport and light emission, allowing electrical programming to define persistently retained optical states. Optimized P‐OLETs exhibit a large memory window of 27.07 V, stable luminance retention over 5000 s, and reliable endurance over 100 program/erase cycles. Floating‐gate charge storage shifts OLET operation from bias‐defined emission toward charge‐state defined emission and establishes a memory‐emission integrated device architecture. This work introduces programmable state‐retentive emission as a compact operating concept for programmable optoelectronics and reconfigurable display systems.

Abstract Image

浮栅电荷存储实现的可编程有机发光晶体管
高分辨率智能手机、可穿戴屏幕和近眼VR/AR微显示器的显示技术越来越需要具有高孔径比的紧凑像素架构。有机发光晶体管(olet)通过在单个器件内结合晶体管开关和电致发光来提高功能集成。然而,传统的oled仍然通过瞬时电偏置来定义发射状态,使状态存储与光发射分离。在基于OLET的像素器件中,存储器-发射共定位的缺失限制了固有状态的可编程性。在这里,我们报告了基于浮栅架构的可编程有机发光晶体管(P‐olet),其中电荷存储实现可逆电荷捕获和释放,产生可编程开关行为和可调谐的电致发光。所述存储电荷调制通道传输和光发射,允许电编程定义持久保留的光态。优化后的P‐olet具有27.07 V的大存储窗口,超过5000 s的稳定亮度保持,以及超过100个程序/擦除周期的可靠耐用性。浮栅电荷存储将OLET操作从偏置定义发射转向电荷状态定义发射,并建立了存储发射集成器件架构。这项工作介绍了可编程状态保持发射作为可编程光电子和可重构显示系统的紧凑操作概念。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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