Francisco J. Pérez-Invernón,Francisco J. Gordillo-Vázquez,Oscar van der Velde,Joan Montanyà,Jesús Alberto López Trujillo,Nicolau Pineda,Diego Loyola,Sora Seo,Christoph Knote,Alexandre O. Fierro,Heidi Huntrieser
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引用次数: 0
Abstract
Lightning is one of the main sources of NO x in the Earth's atmosphere, yet there is considerable variability in NO x production during thunderstorms. In this study, we combined optical lightning data from the Meteosat Third Generation (MTG) Lightning Imaging (LI) instrument, which provides information on the occurrence rate and physical characteristics of lightning flashes, measurements from an extended Lightning Mapping Array (LMA) consisting of 24 sensors, lightning measurements from the Lightning Location System (LLS) of the Meteorological Service of Catalonia (MSC), and TROPOspheric Monitoring Instrument (TROPOMI) cloud and NO 2 research products to investigate lightning NO x emissions in the Ebro Valley (Spain). WRF-Chem simulations were used to calculate the necessary air mass factors and to subtract the NO x not produced by lightning from the TROPOMI measurements, allowing a more accurate estimation of lightning-induced NO x . We found positive relationships between lightning-produced NO x per flash and several lightning properties, including flash channel length, radiance, footprint, duration and the length of the optical continuous signal detected from space. These results highlight the importance of combining detailed lightning observations with atmospheric modeling to quantify NO x emissions from thunderstorms.
期刊介绍:
Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere.
The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.