High-Entropy Engineering to Stabilize Single-Atom Ru Catalysts for Efficient and Durable Water Splitting

IF 17.6 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Angewandte Chemie International Edition Pub Date : 2026-10-15 DOI:10.1002/anie.2676498

Peng-Fei Xie,Yun-Fan Yang,Ju-Zhen Zhang,Binbin He,Feng Zhang,Wenbo Zhao,Peng-Xiang Hou,Yan Sun,Wang Du,Yun Zu,Chang Liu,Yian Wang,Minhua Shao,Jin-Cheng Li

引用次数: 0

Abstract

A high-entropy-engineered strategy to stabilize single Ru atoms on FeCoNiCrMn spinel oxides to overcome the intrinsic activity–stability trade-off, delivering low overpotentials of 280 mV at 100 mA cm−2 for OER and 37 mV at 10 mA cm−2 for HER, a low cell voltage of 1.66 V at 1 A cm−2 for AEMWE and undamped cell performance for 1500 h.

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稳定单原子Ru催化剂的高熵工程用于高效和持久的水裂解

一种高熵工程策略将单个Ru原子稳定在FeCoNiCrMn尖晶石氧化物上，以克服固有活性-稳定性的平衡，为OER提供100 mA cm - 2时280 mV的低过电位，为HER提供10 mA cm - 2时37 mV的低过电位，为AEMWE提供1 A cm - 2时1.66 V的低电池电压和1500小时的无衰减电池性能。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Angewandte Chemie International Edition 化学-化学综合

CiteScore

26.60

自引率

6.60%

发文量

3549

审稿时长

1.5 months

期刊介绍： Angewandte Chemie, a journal of the German Chemical Society (GDCh), maintains a leading position among scholarly journals in general chemistry with an impressive Impact Factor of 16.6 (2022 Journal Citation Reports, Clarivate, 2023). Published weekly in a reader-friendly format, it features new articles almost every day. Established in 1887, Angewandte Chemie is a prominent chemistry journal, offering a dynamic blend of Review-type articles, Highlights, Communications, and Research Articles on a weekly basis, making it unique in the field.