Khurrum Saleem Chaudri, Mohammad Alrwashdeh, Mohamed Lahdour, Antonio Cammi, Saeed A. Alameri
{"title":"Comparative neutronic assessment of U3Si2-based accident-tolerant fuels in a two-batch APR-1400","authors":"Khurrum Saleem Chaudri, Mohammad Alrwashdeh, Mohamed Lahdour, Antonio Cammi, Saeed A. Alameri","doi":"10.1016/j.radphyschem.2026.114509","DOIUrl":null,"url":null,"abstract":"Uranium silicide (U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>) is a leading candidate for accident-tolerant fuel in light-water reactors due to its higher uranium density and superior thermal conductivity compared with conventional UO<ce:inf loc=\"post\">2</ce:inf>. However, its limited oxidation resistance and phase stability under reactor-relevant conditions have motivated the development of alternative designs, including composite and doped fuel architectures. This study presents a comparative neutronic evaluation of several U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>-based fuel concepts for a 24-month APR-1400 equilibrium core using the CASMO4E/SIMULATE3 code system. The CASMO4E/SIMULATE3 calculation route for accident-tolerant fuel analysis is verified against the VERA ATF benchmark, proposed by ORNL. The investigated options include monolithic U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>, homogeneous U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>–UB<ce:inf loc=\"post\">2</ce:inf> composite fuel, Cr-doped U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>, UO<ce:inf loc=\"post\">2</ce:inf>–U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf> composite fuel, and newly proposed multilayer U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf>/UB<ce:inf loc=\"post\">2</ce:inf> configurations using natural boron. These multilayer concepts are introduced to suppress excess reactivity, reduce dependence on costly B-11 enrichment, and, in the outer-layer configuration, limit direct exposure of U<ce:inf loc=\"post\">3</ce:inf>Si<ce:inf loc=\"post\">2</ce:inf> to water or steam.","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"297 1","pages":"114509"},"PeriodicalIF":3.5000,"publicationDate":"2026-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1016/j.radphyschem.2026.114509","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Uranium silicide (U3Si2) is a leading candidate for accident-tolerant fuel in light-water reactors due to its higher uranium density and superior thermal conductivity compared with conventional UO2. However, its limited oxidation resistance and phase stability under reactor-relevant conditions have motivated the development of alternative designs, including composite and doped fuel architectures. This study presents a comparative neutronic evaluation of several U3Si2-based fuel concepts for a 24-month APR-1400 equilibrium core using the CASMO4E/SIMULATE3 code system. The CASMO4E/SIMULATE3 calculation route for accident-tolerant fuel analysis is verified against the VERA ATF benchmark, proposed by ORNL. The investigated options include monolithic U3Si2, homogeneous U3Si2–UB2 composite fuel, Cr-doped U3Si2, UO2–U3Si2 composite fuel, and newly proposed multilayer U3Si2/UB2 configurations using natural boron. These multilayer concepts are introduced to suppress excess reactivity, reduce dependence on costly B-11 enrichment, and, in the outer-layer configuration, limit direct exposure of U3Si2 to water or steam.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.