Nanosecond laser fabricated multi-scale microtextures for enhancing EBCs adhesion on SiC substrates

IF 3 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY
Zhaoyang Zhai, Qiankun Ding, Haoxuan He, Yanchao Zhang, Dongya Zhang, Chunhua Du
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引用次数: 0

Abstract

Spalling failure at the substrate-environmental barrier coatings (EBCs) interface severely limits the service performance of SiC-based components for service in high-temperature water-vapor environments. In this study, nanosecond laser machining was employed to fabricate multi-scale microtextures on the surface of SiC substrates. The influences of texture fraction, texture depth and inner diameter on coating bonding strength were systematically investigated. The underlying interfacial strengthening and failure mechanisms were further clarified based on morphological observations and elemental characterization. The results demonstrate that multi-scale microtextures substantially enlarge the actual interfacial contact area and achieve synergistic strengthening from the combination of mechanical interlocking and interfacial chemical bonding. A relatively high bonding strength is obtained at a texture fraction of 50% with a moderate inner diameter, where full coating-filling and uniform interfacial stress distribution can be achieved simultaneously. Insufficient mechanical interlocking occurs in overly shallow textures, whereas excessively deep textures readily form closed internal pores. Too-small inner diameters hinder coating infiltration; in contrast, overly large inner diameters reduce the effective anchoring depth and aggravate stress concentration. By tuning the interface morphology, laser-fabricated multi-scale microtextures effectively inhibit coating spalling.

纳秒激光在SiC衬底上制备多尺度微结构以增强EBCs的粘附力
衬底-环境屏障涂层(EBCs)界面的剥落破坏严重限制了sic基组件在高温水蒸气环境中的使用性能。在本研究中,采用纳秒激光加工技术在SiC衬底表面制备了多尺度微纹理。系统地研究了织构分数、织构深度和内径对涂层结合强度的影响。基于形态观察和元素表征,进一步阐明了潜在的界面强化和破坏机制。结果表明,多尺度微织构极大地扩大了实际界面接触面积,并通过机械联锁和界面化学键的结合实现了协同强化。当织构分数为50%、内径适中时,可以获得较高的结合强度,同时实现充分的涂层填充和均匀的界面应力分布。在过浅的织构中发生不充分的机械联锁,而过深的织构容易形成封闭的内部孔隙。内径过小阻碍涂层渗入;过大的内径会降低有效锚固深度,加剧应力集中。通过调整界面形态,激光制备的多尺度微织构有效地抑制了涂层的剥落。
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来源期刊
Applied Physics A
Applied Physics A 工程技术-材料科学:综合
CiteScore
4.80
自引率
7.40%
发文量
964
审稿时长
38 days
期刊介绍: Applied Physics A publishes experimental and theoretical investigations in applied physics as regular articles, rapid communications, and invited papers. The distinguished 30-member Board of Editors reflects the interdisciplinary approach of the journal and ensures the highest quality of peer review.
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