Arpan Ghosh, Seema Rani, Anshul Rasyotra, Samriddha Ray, Karthik G. Krishnan, Md Sajjad Alam, Anirban Chowdhury, Kaushik Ghosh, Saptarshi Das
{"title":"Encoding Light in Electronic Noise","authors":"Arpan Ghosh, Seema Rani, Anshul Rasyotra, Samriddha Ray, Karthik G. Krishnan, Md Sajjad Alam, Anirban Chowdhury, Kaushik Ghosh, Saptarshi Das","doi":"10.1021/acsnano.6c08996","DOIUrl":null,"url":null,"abstract":"<p>Optical sensing in semiconductors is traditionally governed\r\nby\r\nphotoconductive, photovoltaic, and photogating effects, in which optical\r\ninputs are encoded as continuous variations in average current. Here,\r\nwe demonstrate a fundamentally distinct paradigm in which light is\r\nencoded in stochastic transport dynamics rather than steady-state\r\nconductance. Using a monolayer MoS<sub>2</sub> field-effect transistor\r\nwith an aggressively scaled gate stack (∼1.3 nm equivalent\r\noxide thickness), we access a regime where interfacial defect states\r\ndominate transport and form gate-tunable potential wells. At low temperature,\r\ncarrier emission from these states is suppressed, stabilizing trapped\r\nconfigurations in the dark, whereas optical excitation selectively\r\nactivates emission, giving rise to large-amplitude (“giant”)\r\nrandom telegraph noise. This enables independent control of capture\r\nand emission processes through electrostatic gating and illumination,\r\nrespectively, creating a direct mapping between optical input and\r\nstochastic observables such as switching rates, dwell times, and state\r\noccupancies. Interestingly, optical detection is achieved through\r\nthe statistics of rare emission events, enabling sensitivity to ultralow\r\nillumination levels (∼50 fW). Spectral dependence further reveals\r\nphoton energy–dependent emission kinetics, confirming the role\r\nof photon-assisted detrapping. These results show a light-induced\r\nnonequilibrium transport regime in which defect-mediated fluctuations,\r\nconventionally treated as noise, act as a functional signal and provide\r\na stochastic sensing framework for ultralow-light detection in nanoscale\r\nelectronic systems.</p>","PeriodicalId":21,"journal":{"name":"ACS Nano","volume":"20 41","pages":"27738–27747"},"PeriodicalIF":17.3000,"publicationDate":"2026-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Nano","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsnano.6c08996","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2026/10/5 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Optical sensing in semiconductors is traditionally governed
by
photoconductive, photovoltaic, and photogating effects, in which optical
inputs are encoded as continuous variations in average current. Here,
we demonstrate a fundamentally distinct paradigm in which light is
encoded in stochastic transport dynamics rather than steady-state
conductance. Using a monolayer MoS2 field-effect transistor
with an aggressively scaled gate stack (∼1.3 nm equivalent
oxide thickness), we access a regime where interfacial defect states
dominate transport and form gate-tunable potential wells. At low temperature,
carrier emission from these states is suppressed, stabilizing trapped
configurations in the dark, whereas optical excitation selectively
activates emission, giving rise to large-amplitude (“giant”)
random telegraph noise. This enables independent control of capture
and emission processes through electrostatic gating and illumination,
respectively, creating a direct mapping between optical input and
stochastic observables such as switching rates, dwell times, and state
occupancies. Interestingly, optical detection is achieved through
the statistics of rare emission events, enabling sensitivity to ultralow
illumination levels (∼50 fW). Spectral dependence further reveals
photon energy–dependent emission kinetics, confirming the role
of photon-assisted detrapping. These results show a light-induced
nonequilibrium transport regime in which defect-mediated fluctuations,
conventionally treated as noise, act as a functional signal and provide
a stochastic sensing framework for ultralow-light detection in nanoscale
electronic systems.
期刊介绍:
ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.