Encoding Light in Electronic Noise

IF 17.3 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
ACS Nano Pub Date : 2026-10-20 Epub Date: 2026-10-05 DOI:10.1021/acsnano.6c08996
Arpan Ghosh, Seema Rani, Anshul Rasyotra, Samriddha Ray, Karthik G. Krishnan, Md Sajjad Alam, Anirban Chowdhury, Kaushik Ghosh, Saptarshi Das
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引用次数: 0

Abstract

Optical sensing in semiconductors is traditionally governed by photoconductive, photovoltaic, and photogating effects, in which optical inputs are encoded as continuous variations in average current. Here, we demonstrate a fundamentally distinct paradigm in which light is encoded in stochastic transport dynamics rather than steady-state conductance. Using a monolayer MoS2 field-effect transistor with an aggressively scaled gate stack (∼1.3 nm equivalent oxide thickness), we access a regime where interfacial defect states dominate transport and form gate-tunable potential wells. At low temperature, carrier emission from these states is suppressed, stabilizing trapped configurations in the dark, whereas optical excitation selectively activates emission, giving rise to large-amplitude (“giant”) random telegraph noise. This enables independent control of capture and emission processes through electrostatic gating and illumination, respectively, creating a direct mapping between optical input and stochastic observables such as switching rates, dwell times, and state occupancies. Interestingly, optical detection is achieved through the statistics of rare emission events, enabling sensitivity to ultralow illumination levels (∼50 fW). Spectral dependence further reveals photon energy–dependent emission kinetics, confirming the role of photon-assisted detrapping. These results show a light-induced nonequilibrium transport regime in which defect-mediated fluctuations, conventionally treated as noise, act as a functional signal and provide a stochastic sensing framework for ultralow-light detection in nanoscale electronic systems.

在电子噪声中编码光
半导体中的光传感传统上由光导、光伏和光门效应控制,其中光输入被编码为平均电流的连续变化。在这里,我们展示了一种根本不同的范式,其中光被编码为随机输运动力学而不是稳态电导。使用具有积极缩放栅极堆叠(约1.3 nm等效氧化物厚度)的单层MoS2场效应晶体管,我们进入了界面缺陷状态主导输运并形成栅极可调谐势阱的区域。在低温下,这些状态的载流子发射被抑制,在黑暗中稳定了被困构型,而光激发选择性地激活了发射,产生了大振幅(“巨大”)随机电报噪声。这使得分别通过静电门控和照明独立控制捕获和发射过程成为可能,从而在光输入和随机可观察物(如开关速率、停留时间和状态占用)之间创建直接映射。有趣的是,光学检测是通过统计罕见的发射事件来实现的,从而实现了对超低照度(~ 50 fW)的灵敏度。光谱依赖性进一步揭示了光子能量依赖性发射动力学,证实了光子辅助脱陷的作用。这些结果显示了光诱导的非平衡输运机制,其中缺陷介导的波动,通常被视为噪声,作为功能信号,并为纳米级电子系统中的超低光检测提供了随机传感框架。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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