{"title":"A systematic approach to Covariance matrix formulation in charged particle activation experiments","authors":"Tanmoy Bar","doi":"10.1016/j.radphyschem.2026.114514","DOIUrl":null,"url":null,"abstract":"This work presents a detailed covariance and correlation matrix analysis for experimentally measured cross sections obtained using the activation technique. Both statistical and systematic contributions to the covariance matrix were explicitly calculated using sensitivity coefficients. The detector efficiency was determined by refitting standard source data with an exponential function, and the associated covariance matrix of the fitted parameters was propagated to estimate the uncertainty in efficiency at the relevant <mml:math altimg=\"si160.svg\" display=\"inline\"><mml:mi>γ</mml:mi></mml:math>-ray energy. The cross sections and the corresponding experimental parameters, such as beam flux, target thickness, <mml:math altimg=\"si160.svg\" display=\"inline\"><mml:mi>γ</mml:mi></mml:math>-ray intensity, and decay corrections, were taken from previously published measurements and are used here for the purpose of illustrating the covariance formalism. The resulting covariance and correlation matrices provide a comprehensive representation of uncertainties and their interdependencies. This formalism demonstrates the importance of including correlated uncertainties for reliable interpretation and comparison of experimental cross section data.","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"402 1","pages":""},"PeriodicalIF":3.5000,"publicationDate":"2026-09-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1016/j.radphyschem.2026.114514","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
This work presents a detailed covariance and correlation matrix analysis for experimentally measured cross sections obtained using the activation technique. Both statistical and systematic contributions to the covariance matrix were explicitly calculated using sensitivity coefficients. The detector efficiency was determined by refitting standard source data with an exponential function, and the associated covariance matrix of the fitted parameters was propagated to estimate the uncertainty in efficiency at the relevant γ-ray energy. The cross sections and the corresponding experimental parameters, such as beam flux, target thickness, γ-ray intensity, and decay corrections, were taken from previously published measurements and are used here for the purpose of illustrating the covariance formalism. The resulting covariance and correlation matrices provide a comprehensive representation of uncertainties and their interdependencies. This formalism demonstrates the importance of including correlated uncertainties for reliable interpretation and comparison of experimental cross section data.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.