Perovskite fluid dynamics

IF 6.3 3区 综合性期刊 Q1 Multidisciplinary
Fundamental Research Pub Date : 2026-09-01 Epub Date: 2025-08-29 DOI:10.1016/j.fmre.2025.08.007
Changshun Chen, Yingdong Xia, Yonghua Chen
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引用次数: 0

Abstract

The phase transition of perovskite thin films is inherently rapid and highly sensitive to multiple factors. Fluid dynamics has emerged as a powerful framework for elucidating the crystallization and phase transformation processes in perovskites. It governs solute transport, energy dissipation pathways, and mass transfer efficiency, thereby exerting a significant influence on nucleation behavior and crystal growth dynamics. These factors are critical for optimizing film morphology and enhancing device performance in large-area perovskite modules. In this perspective, we first explore the regulatory role of fluid dynamics across distinct phase transition stages and the underlying mechanisms. Then, its practical value in improving film uniformity and optoelectronic performance is examined, with particular emphasis on controlling crystal growth orientation and enhancing structural consistency. Such regulation is considered beneficial for improving device performance and ensuring long-term operational stability under ISOS protocols. Finally, we outline emerging opportunities in solution flow control, crystallization induction, defect passivation, and structural design. These insights offer promising directions for addressing key challenges in stability and scalable fabrication, thereby advancing the development of low-cost, manufacturable perovskite technologies.
钙钛矿流体动力学
钙钛矿薄膜的相变具有快速和对多种因素高度敏感的特点。流体动力学已成为阐明钙钛矿结晶和相变过程的有力框架。它控制着溶质输运、能量耗散途径和传质效率,从而对成核行为和晶体生长动力学产生重大影响。这些因素对于优化薄膜形态和提高大面积钙钛矿模块的器件性能至关重要。从这个角度来看,我们首先探讨了流体动力学在不同相变阶段的调节作用和潜在的机制。然后,研究了其在改善薄膜均匀性和光电性能方面的实用价值,特别是在控制晶体生长取向和增强结构一致性方面。这样的规定被认为有利于提高设备性能和确保ISOS协议下的长期运行稳定性。最后,我们概述了在溶液流动控制、结晶诱导、缺陷钝化和结构设计方面出现的机会。这些见解为解决稳定性和可扩展制造方面的关键挑战提供了有希望的方向,从而推动了低成本、可制造的钙钛矿技术的发展。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Fundamental Research
Fundamental Research Multidisciplinary-Multidisciplinary
CiteScore
4.00
自引率
1.60%
发文量
294
审稿时长
79 days
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