Regulation of ultrasonic atomization behavior and preparation of low-melting-point alloy powders

IF 10.2 1区 化学 Q1 ACOUSTICS
Ultrasonics Sonochemistry Pub Date : 2026-10-01 Epub Date: 2026-09-26 DOI:10.1016/j.ultsonch.2026.108082
Xiaofeng Yang, Haodi Li, Dingying Ren, Hao Lan, Xiaoqiang Hu, Qian Wang, Peng Yu
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Abstract

Viscous damping and acoustic radiation pressure challenge the ultrasonic atomization of high-viscosity and high-surface-tension fluids. To address this issue and reveal the underlying mechanisms, a rotational ultrasonic atomization platform was developed. The effects of ultrasonic power, liquid viscosity, horn geometry, rotation speed, and initial momentum on atomization behavior were investigated using high-speed imaging. For low-viscosity liquids, increasing ultrasonic power elevated the Weber number, widened the spray angle from 63 degrees to 142 degrees, and shortened the atomization incubation period from 10.86 s to 8.15 s. For high-viscosity liquids, viscous damping suppressed the capillary wave pathway, making cavitation the dominant mechanism. Driven by the secondary Bjerknes force, cavitation bubbles bridged into branched, neural-network-like clusters. Their collective collapse overcame the viscous dissipation barrier, providing experimental validation for Boguslavskii’s hypothesis. A critical rotation threshold of 60 revolutions per minute was identified. Below this threshold, acoustic pinning confined the liquid on the horn end-face; above it, centrifugal force forcibly thinned the liquid film, triggering atomization. Furthermore, horn geometry determined the atomization onset location, while increased initial momentum accelerated initiation. Experiments on Sn-58Bi melt verified that coupling optimized horn geometry with a centrifugal force field effectively overcomes the surface energy barrier. Based on these findings, a six-stage atomization model is proposed. The capillary wave mechanism primarily achieves initial film thinning by stripping large droplets, while cavitation dominates fine fragmentation. This work systematically investigates the atomization mechanism of high-resistance fluids and demonstrates the fabrication of metal powders via rotational ultrasonic atomization.
超声雾化行为的调控及低熔点合金粉末的制备
粘滞阻尼和声辐射压力对高粘度、高表面张力流体的超声雾化提出了挑战。为了解决这一问题并揭示其潜在机制,开发了一个旋转超声雾化平台。利用高速成像技术研究了超声功率、液体粘度、喇叭几何形状、转速和初始动量对雾化行为的影响。对于低粘度液体,增大超声功率可提高韦伯数,使喷雾角由63°扩大到142°,雾化潜伏期由10.86 s缩短到8.15 s。对于高粘度液体,粘性阻尼抑制毛细波路径,使空化成为主导机制。在次级比约克尼斯力的驱动下,空化气泡桥接成类似神经网络的分支簇。它们的集体坍缩克服了粘性耗散屏障,为Boguslavskii的假设提供了实验验证。确定了每分钟60转的临界旋转阈值。在此阈值以下,声钉钉将液体限制在喇叭端面;在它上面,离心力使液膜变薄,引发雾化。此外,角的几何形状决定了雾化开始的位置,而初始动量的增加加速了起爆。在Sn-58Bi熔体上进行的实验验证了优化的角形与离心力场的耦合可以有效地克服表面能垒。在此基础上,提出了六段雾化模型。毛细波机制主要是通过剥离大液滴来实现初始膜薄化,而空化作用主要是实现细破碎。本文系统地研究了高阻流体的雾化机理,并演示了旋转超声雾化制备金属粉末的方法。
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来源期刊
Ultrasonics Sonochemistry
Ultrasonics Sonochemistry 化学-化学综合
CiteScore
15.80
自引率
11.90%
发文量
361
审稿时长
59 days
期刊介绍: Ultrasonics Sonochemistry stands as a premier international journal dedicated to the publication of high-quality research articles primarily focusing on chemical reactions and reactors induced by ultrasonic waves, known as sonochemistry. Beyond chemical reactions, the journal also welcomes contributions related to cavitation-induced events and processing, including sonoluminescence, and the transformation of materials on chemical, physical, and biological levels. Since its inception in 1994, Ultrasonics Sonochemistry has consistently maintained a top ranking in the "Acoustics" category, reflecting its esteemed reputation in the field. The journal publishes exceptional papers covering various areas of ultrasonics and sonochemistry. Its contributions are highly regarded by both academia and industry stakeholders, demonstrating its relevance and impact in advancing research and innovation.
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