Consistency between zonal mean stratospheric and total column ozone trends (2000–2024)

IF 5.7 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES
Brian Auffarth,Mark Weber,Alexei Rozanov,Carlo Arosio,John P. Burrows,Melanie Coldewey-Egbers,Sean M. Davis,Doug Degenstein,Kimberlee Dubé,Stacey M. Frith,Lucien Froidevaux,Diego Loyola,Vitali E. Fioletov,Viktoria Sofieva,Ronald van der A,Jeannette D. Wild
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Abstract

This study presents an updated assessment of stratospheric and total column ozone trends over the 2000–2024 period using six merged limb-profile datasets and six merged total ozone datasets. Long-term changes were quantified using a multiple linear regression framework that accounts for dynamical and chemical variability. In addition to standard regressors (solar cycle, QBO, ENSO, stratospheric aerosol optical depth), we include Arctic and Antarctic Oscillation indices and the eddy heat flux in each hemisphere as proxies for dynamic variability. Volcanic (and wildfire) aerosol forcing is represented by separate proxies for three periods dominated by the major volcanic events of El Chichón, Pinatubo, and post-2000 volcanic eruptions, including Hunga-Tonga. These period-specific proxies are employed to better account for varying dynamical ozone responses that largely depend on the season and location of the eruptions. All profile datasets consistently show positive trends in the upper stratosphere, with the strongest ozone recovery in southern mid-latitudes, in agreement with other studies. In the lower stratosphere, trends remain weak, spatially heterogeneous, and predominantly negative. A comparison of stratospheric column trends derived from profile data with total ozone trends shows close agreement across all latitude bands. Within the trend uncertainties, total column trends since 2000 are largely driven by stratospheric ozone changes, while tropospheric contributions to zonal-mean total ozone trends (the difference between total and stratospheric column trends) appear negligible. The extended regression framework improves the representation of recent dynamical variability and provides an updated perspective on stratospheric ozone recovery through 2024.
纬向平均平流层和总臭氧柱趋势的一致性(2000-2024)
本研究利用6个合并的边缘剖面数据集和6个合并的臭氧总量数据集,对2000-2024年期间的平流层和总柱臭氧趋势进行了更新评估。长期变化使用多元线性回归框架进行量化,该框架考虑了动态和化学变化。除了标准回归量(太阳周期、QBO、ENSO、平流层气溶胶光学深度)外,我们还包括北极和南极涛动指数以及每个半球的涡旋热通量作为动态变率的代表。火山(和野火)气溶胶强迫由三个时期的单独代用物表示,这三个时期主要是El Chichón、Pinatubo火山事件和2000年后的火山爆发,包括匈牙利-汤加。这些特定时期的代用物被用来更好地解释主要取决于喷发季节和地点的动态臭氧响应的变化。所有剖面资料集一致显示平流层上层有正趋势,在中纬度南部臭氧恢复最强,这与其他研究结果一致。在平流层下层,趋势仍然很弱,在空间上不均匀,而且主要是负的。由剖面资料得出的平流层柱趋势与总臭氧趋势的比较表明,在所有纬度带上都非常一致。在趋势不确定性范围内,2000年以来的总柱趋势主要由平流层臭氧变化驱动,而对流层对纬向平均总臭氧趋势(总柱趋势与平流层柱趋势之间的差异)的贡献似乎可以忽略不计。扩展回归框架改进了近期动态变率的表示,并提供了到2024年平流层臭氧恢复的最新视角。
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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