Pretrained battery transformer (PBT): A foundation model for battery life prediction

IF 30.5 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Ruifeng Tan,Weixiang Hong,Jia Li,Jiaqiang Huang,Tongyi Zhang
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Abstract

Early prediction of battery cycle life is essential for improving battery design, manufacturing and deployment. However, despite encouraging progress with machine learning, battery life prediction remains constrained by scarce data and pronounced heterogeneity across battery chemistries, specifications, formation protocols and operating conditions. Although transfer learning has been widely explored to alleviate these challenges, its effectiveness is limited by the absence of a foundation model that can integrate heterogeneous battery life data and provide broadly useful knowledge for target-scenario specialization. Here we introduce the pretrained battery transformer (PBT), an integrated foundation model comprising a general PBT and specialized PBT models for individual target scenarios. At its core, battery-knowledge-encoded mixture-of-experts layers enable the general PBT to consolidate shared cycling-pattern–lifetime relationships from 13 heterogeneous lithium-ion battery datasets while preserving specialization across distinct aging regimes. The resulting general PBT provides a shared knowledge and parameter foundation from which specialized PBT models are constructed using limited labelled data to capture target-specific degradation behavior. Across 15 downstream datasets covering 977 batteries and 532 aging conditions from lithium-ion, sodium-ion and zinc-ion batteries, the specialized PBT models achieve state-of-the-art performance, outperforming the strongest comparator by 24.8% on average and by up to 73.9%. This study establishes, to our knowledge, the first foundation model for battery life prediction and points towards a shift from isolated, scenario-specific modelling to a reusable knowledge foundation for data-efficient specialization, with broader implications for sustainable-energy prediction problems constrained by scarce and heterogeneous data.
预训练电池变压器(PBT):电池寿命预测的基础模型
电池循环寿命的早期预测对于改进电池的设计、制造和部署至关重要。然而,尽管机器学习取得了令人鼓舞的进展,但电池寿命预测仍然受到数据稀缺和电池化学成分、规格、形成协议和操作条件明显异质性的限制。尽管迁移学习已经被广泛探索以缓解这些挑战,但其有效性受到缺乏基础模型的限制,该模型可以集成异构电池寿命数据并为目标场景专业化提供广泛有用的知识。本文介绍了预训练电池变压器(PBT),这是一个集成的基础模型,包括通用PBT模型和针对单个目标场景的专用PBT模型。在其核心,电池知识编码的混合专家层使通用PBT能够整合来自13个异质锂离子电池数据集的共享循环模式寿命关系,同时保持不同老化机制的专业化。由此产生的通用PBT提供了共享知识和参数基础,利用有限的标记数据构建专门的PBT模型来捕获目标特定的退化行为。在15个下游数据集中,涵盖977个电池和532个锂离子、钠离子和锌离子电池的老化条件,专业的PBT模型达到了最先进的性能,比最强的比较者平均高出24.8%,最高可达73.9%。据我们所知,这项研究建立了电池寿命预测的第一个基础模型,并指出了从孤立的、特定场景的建模到数据高效专业化的可重用知识基础的转变,对受稀缺和异构数据约束的可持续能源预测问题具有更广泛的影响。
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来源期刊
Energy & Environmental Science
Energy & Environmental Science 化学-工程:化工
CiteScore
50.50
自引率
2.20%
发文量
349
审稿时长
2.2 months
期刊介绍: Energy & Environmental Science, a peer-reviewed scientific journal, publishes original research and review articles covering interdisciplinary topics in the (bio)chemical and (bio)physical sciences, as well as chemical engineering disciplines. Published monthly by the Royal Society of Chemistry (RSC), a not-for-profit publisher, Energy & Environmental Science is recognized as a leading journal. It boasts an impressive impact factor of 8.500 as of 2009, ranking 8th among 140 journals in the category "Chemistry, Multidisciplinary," second among 71 journals in "Energy & Fuels," second among 128 journals in "Engineering, Chemical," and first among 181 scientific journals in "Environmental Sciences." Energy & Environmental Science publishes various types of articles, including Research Papers (original scientific work), Review Articles, Perspectives, and Minireviews (feature review-type articles of broad interest), Communications (original scientific work of an urgent nature), Opinions (personal, often speculative viewpoints or hypotheses on current topics), and Analysis Articles (in-depth examination of energy-related issues).
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