Design and numerical analysis of hybrid plasmonic–photonic crystal quantum-dot nanolasers with enhanced spontaneous emission

Nano Trends Pub Date : 2026-09-01 Epub Date: 2026-09-08 DOI:10.1016/j.nwnano.2026.100233
Priyanka, Ravindar Tadi, Ram Soorat
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Abstract

Hybrid plasmonic–photonic crystal cavities offer an attractive paradigm for achieving both ultra-high quality factors and deep subwavelength mode confinement. However, establishing rigorous design rules that balance Purcell enhancement against parasitic non-radiative quenching remains a critical challenge. In this work, we develop a self-consistent multiscale computational framework, validated against analytical and numerical benchmarks, to investigate six hybrid metallic nanoparticle architectures (gold and silver nanospheres, nanorods, and nanostars) integrated into a GaAs L3 photonic crystal cavity coupled to InAs quantum dots. Multi-solver cross-validation between analytical Mie theory, the boundary element method (BEM), and 3D finite-difference time-domain (FDTD) simulations demonstrates close agreement across resonance wavelengths, cross-sections, and field enhancements. We show that the localized density of states (LDOS) and cavity-mode Purcell factors fundamentally decouple for emitter–metal gap distances below 5 nm, where non-radiative Ohmic absorption dominates over radiative decay. Coupling the electrodynamic cavity parameters into semiclassical four-level laser rate equations predicts lasing threshold reductions of up to 85% under the local-response approximation (and over 82% under generalized nonlocal optical response hydrodynamic analysis) for the silver nanorod geometry, driven by optimal longitudinal plasmon resonance alignment at the 900 nm emission wavelength and strong near-field concentration (|E/E0|2≈300). This work provides quantitative design guidelines and operational boundaries for developing high-efficiency, subwavelength hybrid quantum-dot nanolasers.

Abstract Image

增强自发发射等离子体-光子晶体混合量子点纳米激光器的设计与数值分析
等离子体-光子混合晶体腔为实现超高质量因子和深亚波长模式约束提供了一个有吸引力的范例。然而,建立严格的设计规则来平衡Purcell增强和寄生非辐射猝灭仍然是一个关键的挑战。在这项工作中,我们开发了一个自一致的多尺度计算框架,通过分析和数值基准验证,研究了六种混合金属纳米颗粒结构(金和银纳米球,纳米棒和纳米星)集成到耦合到InAs量子点的砷化镓L3光子晶体腔中。解析Mie理论、边界元法(BEM)和三维时域有限差分(FDTD)模拟之间的多求解器交叉验证表明,共振波长、横截面和场增强方面的一致性非常高。我们表明局域态密度(LDOS)和腔模Purcell因子在发射器-金属间隙距离小于5 nm时基本解耦合,其中非辐射欧姆吸收主导辐射衰减。将电动力腔参数耦合到半经典四能级激光速率方程中,预测在900 nm发射波长和强近场浓度(|E/E0|2≈300)下,银纳米棒几何形状的激光阈值在局部响应近似下降低高达85%(在广义非局部光学响应流体动力学分析下降低超过82%)。这项工作为开发高效率、亚波长混合量子点纳米激光器提供了定量设计指导和操作边界。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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