{"title":"Design and numerical analysis of hybrid plasmonic–photonic crystal quantum-dot nanolasers with enhanced spontaneous emission","authors":"Priyanka, Ravindar Tadi, Ram Soorat","doi":"10.1016/j.nwnano.2026.100233","DOIUrl":null,"url":null,"abstract":"<div><div>Hybrid plasmonic–photonic crystal cavities offer an attractive paradigm for achieving both ultra-high quality factors and deep subwavelength mode confinement. However, establishing rigorous design rules that balance Purcell enhancement against parasitic non-radiative quenching remains a critical challenge. In this work, we develop a self-consistent multiscale computational framework, validated against analytical and numerical benchmarks, to investigate six hybrid metallic nanoparticle architectures (gold and silver nanospheres, nanorods, and nanostars) integrated into a GaAs L3 photonic crystal cavity coupled to InAs quantum dots. Multi-solver cross-validation between analytical Mie theory, the boundary element method (BEM), and 3D finite-difference time-domain (FDTD) simulations demonstrates close agreement across resonance wavelengths, cross-sections, and field enhancements. We show that the localized density of states (LDOS) and cavity-mode Purcell factors fundamentally decouple for emitter–metal gap distances below 5 nm, where non-radiative Ohmic absorption dominates over radiative decay. Coupling the electrodynamic cavity parameters into semiclassical four-level laser rate equations predicts lasing threshold reductions of up to 85% under the local-response approximation (and over 82% under generalized nonlocal optical response hydrodynamic analysis) for the silver nanorod geometry, driven by optimal longitudinal plasmon resonance alignment at the 900 nm emission wavelength and strong near-field concentration (<span><math><mrow><msup><mrow><mrow><mo>|</mo><mi>E</mi><mo>/</mo><msub><mrow><mi>E</mi></mrow><mrow><mn>0</mn></mrow></msub><mo>|</mo></mrow></mrow><mrow><mn>2</mn></mrow></msup><mo>≈</mo><mn>300</mn></mrow></math></span>). This work provides quantitative design guidelines and operational boundaries for developing high-efficiency, subwavelength hybrid quantum-dot nanolasers.</div></div>","PeriodicalId":100942,"journal":{"name":"Nano Trends","volume":"15 ","pages":"Article 100233"},"PeriodicalIF":0.0000,"publicationDate":"2026-09-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Trends","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2666978126000577","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2026/9/8 0:00:00","PubModel":"Epub","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
Abstract
Hybrid plasmonic–photonic crystal cavities offer an attractive paradigm for achieving both ultra-high quality factors and deep subwavelength mode confinement. However, establishing rigorous design rules that balance Purcell enhancement against parasitic non-radiative quenching remains a critical challenge. In this work, we develop a self-consistent multiscale computational framework, validated against analytical and numerical benchmarks, to investigate six hybrid metallic nanoparticle architectures (gold and silver nanospheres, nanorods, and nanostars) integrated into a GaAs L3 photonic crystal cavity coupled to InAs quantum dots. Multi-solver cross-validation between analytical Mie theory, the boundary element method (BEM), and 3D finite-difference time-domain (FDTD) simulations demonstrates close agreement across resonance wavelengths, cross-sections, and field enhancements. We show that the localized density of states (LDOS) and cavity-mode Purcell factors fundamentally decouple for emitter–metal gap distances below 5 nm, where non-radiative Ohmic absorption dominates over radiative decay. Coupling the electrodynamic cavity parameters into semiclassical four-level laser rate equations predicts lasing threshold reductions of up to 85% under the local-response approximation (and over 82% under generalized nonlocal optical response hydrodynamic analysis) for the silver nanorod geometry, driven by optimal longitudinal plasmon resonance alignment at the 900 nm emission wavelength and strong near-field concentration (). This work provides quantitative design guidelines and operational boundaries for developing high-efficiency, subwavelength hybrid quantum-dot nanolasers.