{"title":"Reference gap technique in viscoelestic sphere impact modeling.","authors":"Xiaoyan Ye, Yingnan Xiu","doi":"10.1039/d6sm00384b","DOIUrl":null,"url":null,"abstract":"<p><p>Hydrogel spheres, which undergo large deformations under external force, are widely used in applications ranging from soil conservation to biomedicine, soft robotics, and wearable devices. These large deformations induce strong nonlinearities and emergent phenomena, such as collective granular jamming, which remain difficult to capture within a unified numerical framework. In this study, we propose a discrete-continuous model incorporating a reference gap to construct a continuum hydrogel sphere with tunable Young's modulus. When elastic and surface energies become comparable, surface tension is explicitly incorporated into the model. Then, the relationship between the macroscopic Young's modulus and the microscopic stiffness coefficient is established by quasi-static compression of hydrogel spheres and isotropic compression of rectangular hydrogel blocks. We further evaluate the dynamic behavior of hydrogel spheres with Young's modulus <i>Y</i> ranging from 100 Pa to 50 000 Pa and a Poisson's ratio of 0.5, impacting a rigid substrate at velocities ranging from 0.5 m s<sup>-1</sup> to 4.5 m s<sup>-1</sup>, and validate the results against experimental observations. The evolution of morphology and spreading diameter of the superelastic hydrogel spheres, as well as the forces and stresses exerted on spheres, are investigated. The simulation results demonstrate a transition in contact morphology from point contact to Hertzian contact, and eventually to global deformation, accompanied by a corresponding evolution in stress distribution, from point like concentration to single-ring and multi-ring patterns. These phenomena are governed by the propagation of mechanical waves and are characterized by elastic-capillary Mach numbers corresponding to supersonic, critical, subcritical, and highly low subcritical regimes.</p>","PeriodicalId":103,"journal":{"name":"Soft Matter","volume":" ","pages":"6272-6284"},"PeriodicalIF":2.9000,"publicationDate":"2026-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Soft Matter","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1039/d6sm00384b","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Hydrogel spheres, which undergo large deformations under external force, are widely used in applications ranging from soil conservation to biomedicine, soft robotics, and wearable devices. These large deformations induce strong nonlinearities and emergent phenomena, such as collective granular jamming, which remain difficult to capture within a unified numerical framework. In this study, we propose a discrete-continuous model incorporating a reference gap to construct a continuum hydrogel sphere with tunable Young's modulus. When elastic and surface energies become comparable, surface tension is explicitly incorporated into the model. Then, the relationship between the macroscopic Young's modulus and the microscopic stiffness coefficient is established by quasi-static compression of hydrogel spheres and isotropic compression of rectangular hydrogel blocks. We further evaluate the dynamic behavior of hydrogel spheres with Young's modulus Y ranging from 100 Pa to 50 000 Pa and a Poisson's ratio of 0.5, impacting a rigid substrate at velocities ranging from 0.5 m s-1 to 4.5 m s-1, and validate the results against experimental observations. The evolution of morphology and spreading diameter of the superelastic hydrogel spheres, as well as the forces and stresses exerted on spheres, are investigated. The simulation results demonstrate a transition in contact morphology from point contact to Hertzian contact, and eventually to global deformation, accompanied by a corresponding evolution in stress distribution, from point like concentration to single-ring and multi-ring patterns. These phenomena are governed by the propagation of mechanical waves and are characterized by elastic-capillary Mach numbers corresponding to supersonic, critical, subcritical, and highly low subcritical regimes.
水凝胶球在外力作用下发生大变形,广泛应用于土壤保护、生物医学、软机器人和可穿戴设备等领域。这些大变形引起强烈的非线性和紧急现象,如集体颗粒干扰,这仍然难以在统一的数值框架内捕获。在这项研究中,我们提出了一个包含参考间隙的离散-连续模型来构建具有可调杨氏模量的连续水凝胶球。当弹性能和表面能变得可比时,表面张力被明确地纳入模型。然后,通过水凝胶球的准静态压缩和矩形水凝胶块的各向同性压缩,建立了宏观杨氏模量与微观刚度系数之间的关系。我们进一步评估了杨氏模量Y范围为100 Pa至50 000 Pa,泊松比为0.5的水凝胶球在0.5 m s-1至4.5 m s-1的速度下对刚性衬底的影响,并根据实验观察验证了结果。研究了超弹性水凝胶球的形态和直径的演变,以及施加在球上的力和应力。模拟结果表明,接触形态发生了从点接触到赫兹接触,再到全局变形的转变,应力分布也相应发生了从点状集中到单环和多环的演变。这些现象是由机械波的传播所控制的,并以与超音速、临界、亚临界和极低亚临界状态相对应的弹性毛细马赫数为特征。
期刊介绍:
Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.