Qi Wang, Xiaoliang Wang, Haitao Zhai, Yunfei Xie, Yao Bai
{"title":"Comprehensive prediction model for NOx concentration at the SNCR outlet during rapid load fluctuations","authors":"Qi Wang, Xiaoliang Wang, Haitao Zhai, Yunfei Xie, Yao Bai","doi":"10.1002/cjce.70344","DOIUrl":null,"url":null,"abstract":"<p>To address the issues of untimely and unstable control during rapid load fluctuations in the selective non-catalytic reduction (SNCR) denitrification systems at thermal power plants, which lead to potential exceedances of pollutant emission limits, this study proposes a comprehensive predictive model to forecast NO<sub>x</sub> emission concentrations at the system outlet. Firstly, raw data collected from industrial sites undergoes filtering and noise reduction. The multi-dimensional time series is then dynamically calibrated and reduced in dimension utilizing the maximum information coefficient (MIC). Subsequently, combining the advantages of feature extraction and fusion from cross-attention, differential convolutions, and long short-term memory (LSTM) gating, this study proposes a deep integration architecture and introduces a multi-angle improved crested porcupine optimizer (ICPO) algorithm to optimize network hyperparameters adaptively. This approach enhances the model's expressive capability while minimizing computational complexity. Experimental results based on operational data from a 350 MW supercritical circulating fluidized bed (CFB) boiler in a thermal power plant demonstrate that the proposed model outperforms comparison models under various operating conditions, accurately predicting NO<sub>x</sub> emission concentrations at the SNCR outlet.</p>","PeriodicalId":9400,"journal":{"name":"Canadian Journal of Chemical Engineering","volume":"104 9","pages":"4613-4629"},"PeriodicalIF":2.2000,"publicationDate":"2026-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Canadian Journal of Chemical Engineering","FirstCategoryId":"5","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/cjce.70344","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2026/3/23 0:00:00","PubModel":"Epub","JCR":"Q3","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
To address the issues of untimely and unstable control during rapid load fluctuations in the selective non-catalytic reduction (SNCR) denitrification systems at thermal power plants, which lead to potential exceedances of pollutant emission limits, this study proposes a comprehensive predictive model to forecast NOx emission concentrations at the system outlet. Firstly, raw data collected from industrial sites undergoes filtering and noise reduction. The multi-dimensional time series is then dynamically calibrated and reduced in dimension utilizing the maximum information coefficient (MIC). Subsequently, combining the advantages of feature extraction and fusion from cross-attention, differential convolutions, and long short-term memory (LSTM) gating, this study proposes a deep integration architecture and introduces a multi-angle improved crested porcupine optimizer (ICPO) algorithm to optimize network hyperparameters adaptively. This approach enhances the model's expressive capability while minimizing computational complexity. Experimental results based on operational data from a 350 MW supercritical circulating fluidized bed (CFB) boiler in a thermal power plant demonstrate that the proposed model outperforms comparison models under various operating conditions, accurately predicting NOx emission concentrations at the SNCR outlet.
期刊介绍:
The Canadian Journal of Chemical Engineering (CJChE) publishes original research articles, new theoretical interpretation or experimental findings and critical reviews in the science or industrial practice of chemical and biochemical processes. Preference is given to papers having a clearly indicated scope and applicability in any of the following areas: Fluid mechanics, heat and mass transfer, multiphase flows, separations processes, thermodynamics, process systems engineering, reactors and reaction kinetics, catalysis, interfacial phenomena, electrochemical phenomena, bioengineering, minerals processing and natural products and environmental and energy engineering. Papers that merely describe or present a conventional or routine analysis of existing processes will not be considered.