Comprehensive prediction model for NOx concentration at the SNCR outlet during rapid load fluctuations

IF 2.2 4区 工程技术 Q3 ENGINEERING, CHEMICAL
Canadian Journal of Chemical Engineering Pub Date : 2026-08-06 Epub Date: 2026-03-23 DOI:10.1002/cjce.70344
Qi Wang, Xiaoliang Wang, Haitao Zhai, Yunfei Xie, Yao Bai
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引用次数: 0

Abstract

To address the issues of untimely and unstable control during rapid load fluctuations in the selective non-catalytic reduction (SNCR) denitrification systems at thermal power plants, which lead to potential exceedances of pollutant emission limits, this study proposes a comprehensive predictive model to forecast NOx emission concentrations at the system outlet. Firstly, raw data collected from industrial sites undergoes filtering and noise reduction. The multi-dimensional time series is then dynamically calibrated and reduced in dimension utilizing the maximum information coefficient (MIC). Subsequently, combining the advantages of feature extraction and fusion from cross-attention, differential convolutions, and long short-term memory (LSTM) gating, this study proposes a deep integration architecture and introduces a multi-angle improved crested porcupine optimizer (ICPO) algorithm to optimize network hyperparameters adaptively. This approach enhances the model's expressive capability while minimizing computational complexity. Experimental results based on operational data from a 350 MW supercritical circulating fluidized bed (CFB) boiler in a thermal power plant demonstrate that the proposed model outperforms comparison models under various operating conditions, accurately predicting NOx emission concentrations at the SNCR outlet.

负荷快速波动时SNCR出口NOx浓度综合预测模型
针对火力发电厂选择性非催化还原(SNCR)脱硝系统负荷快速波动时控制不及时、控制不稳定导致污染物排放限值超标的问题,本研究提出了一种综合预测模型,对系统出口NOx排放浓度进行预测。首先,从工业场地收集的原始数据经过过滤和降噪。然后利用最大信息系数(MIC)对多维时间序列进行动态校准和降维。随后,结合交叉注意、微分卷积和长短期记忆(LSTM)门控的特征提取和融合优势,提出了深度集成架构,并引入了多角度改进的冠猪优化器(ICPO)算法对网络超参数进行自适应优化。这种方法增强了模型的表达能力,同时最小化了计算复杂度。基于某火电厂350mw超临界循环流化床(CFB)锅炉运行数据的实验结果表明,该模型在各种运行条件下均优于对比模型,能够准确预测SNCR出口NOx排放浓度。
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来源期刊
Canadian Journal of Chemical Engineering
Canadian Journal of Chemical Engineering 工程技术-工程:化工
CiteScore
3.60
自引率
14.30%
发文量
448
审稿时长
3.2 months
期刊介绍: The Canadian Journal of Chemical Engineering (CJChE) publishes original research articles, new theoretical interpretation or experimental findings and critical reviews in the science or industrial practice of chemical and biochemical processes. Preference is given to papers having a clearly indicated scope and applicability in any of the following areas: Fluid mechanics, heat and mass transfer, multiphase flows, separations processes, thermodynamics, process systems engineering, reactors and reaction kinetics, catalysis, interfacial phenomena, electrochemical phenomena, bioengineering, minerals processing and natural products and environmental and energy engineering. Papers that merely describe or present a conventional or routine analysis of existing processes will not be considered.
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