{"title":"A Physics-Based Reduced-Order Model to Predict Gas Holdup in Bubble Columns","authors":"Vamsi Pyla, Racha Varun Kumar, Varun Shastry, Aditya Singh, Himanshu Goyal","doi":"10.1021/acsengineeringau.5c00101","DOIUrl":null,"url":null,"abstract":"<p>Bubble columns are extensively used in the process industry\r\nfor\r\ngas–liquid contact operations. The Euler–Euler CFD model\r\nis commonly used to simulate bubble columns. However, the high computational\r\ncost of these simulations makes them impractical for rapid design-space\r\nexploration. Consequently, bubble column design relies heavily on\r\nempirical correlations, which have limited generalizability and predictive\r\naccuracy. To address this limitation, a physics-based reduced-order\r\nmodel (ROM) is developed via cross-sectional averaging of the Euler–Euler\r\ngas and liquid phase continuity and momentum conservation equations.\r\nThe developed ROM consists of five algebraic equations without any\r\ntuning parameters. The unclosed terms appearing in the ROM are analyzed\r\nand closed using 3D Euler–Euler CFD simulations of bubble column\r\nexperiments. The ROM can predict the overall gas holdup and the cross-sectionally\r\naveraged gas and liquid velocities within seconds. The model’s\r\naccuracy is evaluated against several experiments from the literature,\r\ncovering a wide range of designs (e.g., column diameter, aspect ratio,\r\nand orifice size) and inlet gas velocity (0.01 to 0.2 m/s). The developed\r\nROM outperforms existing empirical correlations in predicting the\r\ngas holdup for Weber number <em>We</em> < 2.</p>","PeriodicalId":29804,"journal":{"name":"ACS Engineering Au","volume":"6 2","pages":"345–358"},"PeriodicalIF":9.0000,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Engineering Au","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsengineeringau.5c00101","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2026/1/26 0:00:00","PubModel":"Epub","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Bubble columns are extensively used in the process industry
for
gas–liquid contact operations. The Euler–Euler CFD model
is commonly used to simulate bubble columns. However, the high computational
cost of these simulations makes them impractical for rapid design-space
exploration. Consequently, bubble column design relies heavily on
empirical correlations, which have limited generalizability and predictive
accuracy. To address this limitation, a physics-based reduced-order
model (ROM) is developed via cross-sectional averaging of the Euler–Euler
gas and liquid phase continuity and momentum conservation equations.
The developed ROM consists of five algebraic equations without any
tuning parameters. The unclosed terms appearing in the ROM are analyzed
and closed using 3D Euler–Euler CFD simulations of bubble column
experiments. The ROM can predict the overall gas holdup and the cross-sectionally
averaged gas and liquid velocities within seconds. The model’s
accuracy is evaluated against several experiments from the literature,
covering a wide range of designs (e.g., column diameter, aspect ratio,
and orifice size) and inlet gas velocity (0.01 to 0.2 m/s). The developed
ROM outperforms existing empirical correlations in predicting the
gas holdup for Weber number We < 2.
期刊介绍:
)ACS Engineering Au is an open access journal that reports significant advances in chemical engineering applied chemistry and energy covering fundamentals processes and products. The journal's broad scope includes experimental theoretical mathematical computational chemical and physical research from academic and industrial settings. Short letters comprehensive articles reviews and perspectives are welcome on topics that include:Fundamental research in such areas as thermodynamics transport phenomena (flow mixing mass & heat transfer) chemical reaction kinetics and engineering catalysis separations interfacial phenomena and materialsProcess design development and intensification (e.g. process technologies for chemicals and materials synthesis and design methods process intensification multiphase reactors scale-up systems analysis process control data correlation schemes modeling machine learning Artificial Intelligence)Product research and development involving chemical and engineering aspects (e.g. catalysts plastics elastomers fibers adhesives coatings paper membranes lubricants ceramics aerosols fluidic devices intensified process equipment)Energy and fuels (e.g. pre-treatment processing and utilization of renewable energy resources; processing and utilization of fuels; properties and structure or molecular composition of both raw fuels and refined products; fuel cells hydrogen batteries; photochemical fuel and energy production; decarbonization; electrification; microwave; cavitation)Measurement techniques computational models and data on thermo-physical thermodynamic and transport properties of materials and phase equilibrium behaviorNew methods models and tools (e.g. real-time data analytics multi-scale models physics informed machine learning models machine learning enhanced physics-based models soft sensors high-performance computing)