Degradation Prediction of Proton-Exchange Membrane Fuel Cell Tested Under Static and Quasi-Dynamic Operating Conditions

IF 3.1 4区 工程技术 Q3 ELECTROCHEMISTRY
Fuel Cells Pub Date : 2026-06-07 DOI:10.1002/fuce.70116
Matthew Georgio Dekkers, Marcia L. Baptista, Helmut Prendinger
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Abstract

The viability and extended lifetime of proton-exchange membrane (PEM) fuel cells are essential to enable hydrogen electric aviation. Their reliability, that is, the ability to maintain stable performance over long operational periods under varying environmental and load conditions, is a critical factor for their adoption in aviation systems. Prognostics and Health Management (PHM) is a popular strategy used extensively in aero engines. This data-driven approach is used to estimate the best maintenance times and to prevent utilisation of equipment beyond its end-of-life. Despite being considerably well established in classical aeronautics, PHM is not yet mature for PEM fuel cells. Currently PHM for PEM fuel cells face three technical problems: (1) reliance on multi-sensor datasets that limit applicability when only voltage and current measurements are available, (2) short-term prediction windows of typically below 100 h, and (3) limited linkage between physics models and machine learning models for RUL predictions. This study presents a hybrid long short-term memory (LSTM) and echo state network (ESN) framework to address gaps (1) and (2) under static and quasi-dynamic conditions. Using seasonal and trend decomposition using LOESS (STL), voltage and current are separated into components, enabling medium-term prediction up to 125 h. Existing membrane degradation models are utilised to establish a foundation for future linkage with a machine learning model to improve remaining useful life (RUL) predictions. Our results suggest that the hybrid LSTM–ESN framework enables 125-h degradation predictions using only voltage and current measurements.

Abstract Image

静态和准动态工况下质子交换膜燃料电池的降解预测
质子交换膜(PEM)燃料电池的生存能力和延长的使用寿命对氢动力航空至关重要。它们的可靠性,即在不同环境和负载条件下长时间保持稳定性能的能力,是航空系统采用它们的关键因素。预测和健康管理(PHM)是一种广泛应用于航空发动机的策略。这种数据驱动的方法用于估计最佳维护时间,并防止设备超过其使用寿命。尽管PHM在经典航空学中已经相当成熟,但用于PEM燃料电池的PHM还不成熟。目前PEM燃料电池的PHM面临三个技术问题:(1)依赖于多传感器数据集,当只有电压和电流测量可用时,其适用性受到限制;(2)短期预测窗口通常低于100小时;(3)物理模型和机器学习模型之间的联系有限,无法用于RUL预测。本研究提出了一种长短期记忆(LSTM)和回声状态网络(ESN)混合框架,以解决静态和准动态条件下的差距(1)和(2)。使用黄土(STL)进行季节和趋势分解,将电压和电流分离成组件,实现长达125小时的中期预测。利用现有的膜降解模型为未来与机器学习模型的联系奠定基础,以提高剩余使用寿命(RUL)预测。我们的研究结果表明,混合LSTM-ESN框架仅使用电压和电流测量就可以实现125小时的退化预测。
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来源期刊
Fuel Cells
Fuel Cells 工程技术-电化学
CiteScore
5.80
自引率
3.60%
发文量
31
审稿时长
3.7 months
期刊介绍: This journal is only available online from 2011 onwards. Fuel Cells — From Fundamentals to Systems publishes on all aspects of fuel cells, ranging from their molecular basis to their applications in systems such as power plants, road vehicles and power sources in portables. Fuel Cells is a platform for scientific exchange in a diverse interdisciplinary field. All related work in -chemistry- materials science- physics- chemical engineering- electrical engineering- mechanical engineering- is included. Fuel Cells—From Fundamentals to Systems has an International Editorial Board and Editorial Advisory Board, with each Editor being a renowned expert representing a key discipline in the field from either a distinguished academic institution or one of the globally leading companies. Fuel Cells—From Fundamentals to Systems is designed to meet the needs of scientists and engineers who are actively working in the field. Until now, information on materials, stack technology and system approaches has been dispersed over a number of traditional scientific journals dedicated to classical disciplines such as electrochemistry, materials science or power technology. Fuel Cells—From Fundamentals to Systems concentrates on the publication of peer-reviewed original research papers and reviews.
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