Self-powered sucrose detection using a superhydrophobic liquid–solid triboelectric nanogenerator

IF 8.1 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Premkumar Sharad Bhosale, Sugato Hajra, Swati Panda, Kushal Ruthvik Kaja, Mohamed Belal, Soon Moon Jeong and Hoe Joon Kim
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Abstract

Real-time monitoring of sucrose concentration is essential in intelligent industrial processing, food quality control, and biochemical manufacturing, creating demand for sustainable and autonomous sensing technologies. In this work, a liquid–solid triboelectric nanogenerator (LS-TENG) is developed for simultaneous energy harvesting and sucrose concentration sensing using deionized water (DI) and sucrose solutions as the active liquid medium. The device employs a hydrophobic polytetrafluoroethylene (PTFE) surface as the solid triboelectric layer, enabling repeated charge generation during droplet contact–separation events. Changes in sucrose concentration significantly affect charge density and electrical output, enabling quantitative sensing without external power sources. The developed LS-TENG achieves a maximum output voltage of −37 V and a current of 52 nA, demonstrating efficient conversion of droplet kinetic energy into electrical signals. The sensing mechanism is attributed to sucrose-induced disruption of the hydrogen-bonding network of water, forming sucrose–water interactions that alter solution conductivity and flow behavior. This study introduces a sustainable, self-powered triboelectric sensing probe, offering a promising platform for real-time sucrose monitoring in smart industrial and process-control applications.

Abstract Image

使用超疏水液-固摩擦电纳米发电机的自供电蔗糖检测
蔗糖浓度的实时监测在智能工业加工、食品质量控制和生化制造中至关重要,这创造了对可持续和自主传感技术的需求。在这项工作中,开发了一种液-固摩擦电纳米发电机(LS-TENG),以去离子水(DI)和蔗糖溶液作为活性液体介质,同时进行能量收集和蔗糖浓度传感。该装置采用疏水性聚四氟乙烯(PTFE)表面作为固体摩擦电层,在液滴接触分离事件中可以重复产生电荷。蔗糖浓度的变化显著影响电荷密度和电输出,无需外部电源即可实现定量传感。研制的LS-TENG最大输出电压为- 37 V,电流为52 nA,能够有效地将液滴动能转化为电信号。该传感机制归因于蔗糖诱导水的氢键网络的破坏,形成蔗糖-水相互作用,改变溶液的导电性和流动行为。本研究介绍了一种可持续的、自供电的摩擦电传感探头,为智能工业和过程控制应用中的实时蔗糖监测提供了一个有前途的平台。
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来源期刊
Materials Chemistry Frontiers
Materials Chemistry Frontiers Materials Science-Materials Chemistry
CiteScore
12.00
自引率
2.90%
发文量
313
期刊介绍: Materials Chemistry Frontiers focuses on the synthesis and chemistry of exciting new materials, and the development of improved fabrication techniques. Characterisation and fundamental studies that are of broad appeal are also welcome. This is the ideal home for studies of a significant nature that further the development of organic, inorganic, composite and nano-materials.
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