Microfluidic Investigation of High-Pressure High-Temperature Pore-Scale Hydrocarbon Gas–Water–Oil Three-Phase Flow in Reservoir-Type Underground Gas Storage

IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL
Qian Zhang, Dewen Zheng, Jieming Wang, Lei Shi, Chun Li, Huayin Zhu
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Abstract

Understanding pore-scale hydrocarbon gas–water–oil three-phase flow in reservoir-type underground gas storage (UGS) remains limited, particularly under repeated seasonal injection-withdrawal cycles at elevated pressure and temperature. This gap limits mechanistic interpretation of injectivity evolution, pressure hysteresis, and working-gas loss in oil reservoirs converted to UGS. The present study develops an HPHT microfluidic visualization platform to observe three-phase dynamics in a sandstone-pattern micromodel at 85 °C under cyclic pressures of 10–29 MPa. The protocol reproduces key stages of UGS construction and operation, enabling real-time tracking of interfaces, phase redistribution, and connectivity. Weakly water-wet/mixed-wet conditions create persistent capillary heterogeneity, leading to capillarity-controlled fingering, snap-off, and immobilized oil films and ganglia during waterflooding, which subsequently constrain gas accessibility. During graded gas injection, intermittent pore-scale invasions and gas–water reconfiguration rapidly establish preferential gas pathways that dominate injectivity and cushion-gas development. Concurrently, sustained gas–oil contact promotes interphase mass transfer (gas dissolution into oil), manifested by oil swelling and enhanced oil mobility that locally assists remobilization and pathway evolution along the pressure trajectory. During withdrawal, wetting-phase re-imbibition partially collapses gas pathways, while flow reversal induces interfacial shear that redistributes wall-attached liquid films, together promoting irreversible gas trapping and connectivity hysteresis. In the first cycle, bulk gas saturation increases from ~ 40 to ~ 72%, while oil displacement efficiency (used solely as a diagnostic for three-phase redistribution) rises from ~ 12 to ~ 23% during injection and reaches ~ 26–27% at early withdrawal. These pore-scale observations provide mechanistic constraints for optimizing pressure windows and maximizing working-gas recovery in reservoir-type UGS systems.

储层型地下储气库高压高温孔隙尺度烃类气-水-油三相流动的微流体研究
对储层型地下储气库(UGS)孔隙级油气气水油三相流动的理解仍然有限,特别是在高压高温下反复的季节性注入-回收循环下。这一差距限制了对UGS油藏注入演化、压力滞后和工作气损失的机理解释。本研究开发了一个HPHT微流控可视化平台,用于观察85℃下10-29 MPa循环压力下砂岩型微模型的三相动力学。该协议再现了UGS构建和运行的关键阶段,实现了接口的实时跟踪、相位重新分配和连接。弱水湿/混湿条件会造成持续的毛细非均质性,导致水驱过程中毛细控制的指动、断裂、油膜和神经节的固定,从而限制了天然气的可及性。在分级注气过程中,间歇性孔隙尺度侵入和气水重构迅速建立了优先气路,主导了注入和缓冲气开发。同时,持续的油气接触促进了相间传质(气体溶解到油中),表现为油的膨胀和油的流动性增强,局部有助于再动员和沿压力轨迹的路径演化。在回采过程中,润湿相的再吸胀使气体通道部分崩溃,而流动逆转引起界面剪切,重新分配附着在壁面的液膜,共同促进不可逆气体捕获和连通性滞后。在第一个循环中,整体气饱和度从~ 40%增加到~ 72%,而驱油效率(仅用于三相再分配的诊断)在注入期间从~ 12%上升到~ 23%,在早期退出时达到~ 26-27%。这些孔隙尺度的观察结果为优化压力窗口和最大化储层型UGS系统的工作气采收率提供了机制约束。
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来源期刊
Transport in Porous Media
Transport in Porous Media 工程技术-工程:化工
CiteScore
5.30
自引率
7.40%
发文量
155
审稿时长
4.2 months
期刊介绍: -Publishes original research on physical, chemical, and biological aspects of transport in porous media- Papers on porous media research may originate in various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering)- Emphasizes theory, (numerical) modelling, laboratory work, and non-routine applications- Publishes work of a fundamental nature, of interest to a wide readership, that provides novel insight into porous media processes- Expanded in 2007 from 12 to 15 issues per year. Transport in Porous Media publishes original research on physical and chemical aspects of transport phenomena in rigid and deformable porous media. These phenomena, occurring in single and multiphase flow in porous domains, can be governed by extensive quantities such as mass of a fluid phase, mass of component of a phase, momentum, or energy. Moreover, porous medium deformations can be induced by the transport phenomena, by chemical and electro-chemical activities such as swelling, or by external loading through forces and displacements. These porous media phenomena may be studied by researchers from various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering).
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