A New Framework for Medium- to Long-Term PM2.5 Predictions Using AI-Based High-Resolution Meteorological Forecasts

IF 8.4
Chem & Bio Engineering Pub Date : 2026-02-26 Epub Date: 2025-12-09 DOI:10.1021/cbe.5c00074
Haonan Gu, Yichao Xu, Hua Pan, Yao Shi, Chunlei Wei, Xiaoyong Cao, Yi He
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引用次数: 0

Abstract

Accurate forecasting of PM2.5 concentrations is vital for effective air quality management and public health protection, particularly in the context of medium- to long-term planning. Such forecasts are also essential for guiding emission control and timely responses in urban and regional environments. Reliable prediction over extended horizons critically depends on access to accurate, high-resolution meteorological fields. To address limitations in traditional approaches that rely on short-term site-level observations or retrospective meteorological fields, this study proposes a deep learning framework that couples AI-based gridded meteorological forecasts with a dynamic graph-based architecture for PM2.5 prediction. The model captures evolving spatiotemporal patterns of pollutant transport and enables extended-range forecasts. By leveraging gridded meteorological forecasts, the proposed framework reduces 3-day RMSE and MAE of the prediction by 12% compared to models without the gridded inputs. For seasonal 10-day forecasts, errors can be decreased by approximately 20% relative to the physics-based Weather Research and Forecasting (WRF)-Community Multiscale Air Quality (CMAQ) system. Furthermore, interpretability analysis reveals the importance of wind-driven spatial asymmetries and supports the design of boundary-aware graph construction. Additional evaluations using Integrated Forecasting System (IFS) and PanGu-Weather forecasts further demonstrate that the model maintains high performance across different gridded data sources without retraining, highlighting its flexibility and potential to incorporate other AI-based meteorological models for adaptable and effective air quality forecasting. These findings underscore the potential of the proposed framework to serve as a computationally efficient and operationally feasible alternative to conventional chemical transport models in future air quality management systems, particularly for early warning systems and targeted emission control strategies.

基于人工智能的高分辨率气象预报中长期PM2.5预测新框架
准确预测PM2.5浓度对于有效的空气质量管理和公众健康保护至关重要,特别是在中长期规划的背景下。这种预报对于指导城市和区域环境中的排放控制和及时反应也是必不可少的。长期可靠的预报关键取决于能否获得准确、高分辨率的气象场。为了解决依赖短期站点级观测或回顾性气象领域的传统方法的局限性,本研究提出了一个深度学习框架,将基于人工智能的网格气象预报与基于动态图形的PM2.5预测架构相结合。该模型捕捉污染物运移的不断演变的时空模式,并能够进行扩展范围的预测。通过利用网格化气象预报,与没有网格化输入的模式相比,所提出的框架将预测的3天RMSE和MAE降低了12%。对于季节性10天预报,相对于基于物理的天气研究与预报(WRF)-社区多尺度空气质量(CMAQ)系统,误差可减少约20%。此外,可解释性分析揭示了风驱动空间不对称的重要性,并为边界感知图构造的设计提供了支持。利用综合预报系统(IFS)和PanGu-Weather预报进行的额外评估进一步表明,该模型无需再训练就能在不同网格数据源中保持高性能,突出了其灵活性和潜力,可将其他基于人工智能的气象模型纳入适应性强且有效的空气质量预报。这些发现强调了所提议的框架在未来的空气质量管理系统中,特别是在早期预警系统和有针对性的排放控制战略中,作为一种计算效率高、操作可行的替代传统化学输送模型的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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