Haonan Gu, Yichao Xu, Hua Pan, Yao Shi, Chunlei Wei, Xiaoyong Cao, Yi He
{"title":"A New Framework for Medium- to Long-Term PM2.5 Predictions Using AI-Based High-Resolution Meteorological Forecasts","authors":"Haonan Gu, Yichao Xu, Hua Pan, Yao Shi, Chunlei Wei, Xiaoyong Cao, Yi He","doi":"10.1021/cbe.5c00074","DOIUrl":null,"url":null,"abstract":"<p>Accurate forecasting of PM<sub>2.5</sub> concentrations\r\nis vital\r\nfor effective air quality management and public health protection,\r\nparticularly in the context of medium- to long-term planning. Such\r\nforecasts are also essential for guiding emission control and timely\r\nresponses in urban and regional environments. Reliable prediction\r\nover extended horizons critically depends on access to accurate, high-resolution\r\nmeteorological fields. To address limitations in traditional approaches\r\nthat rely on short-term site-level observations or retrospective meteorological\r\nfields, this study proposes a deep learning framework that couples\r\nAI-based gridded meteorological forecasts with a dynamic graph-based\r\narchitecture for PM<sub>2.5</sub> prediction. The model captures evolving\r\nspatiotemporal patterns of pollutant transport and enables extended-range\r\nforecasts. By leveraging gridded meteorological forecasts, the proposed\r\nframework reduces 3-day RMSE and MAE of the prediction by 12% compared\r\nto models without the gridded inputs. For seasonal 10-day forecasts,\r\nerrors can be decreased by approximately 20% relative to the physics-based\r\nWeather Research and Forecasting (WRF)-Community Multiscale Air Quality\r\n(CMAQ) system. Furthermore, interpretability analysis reveals the\r\nimportance of wind-driven spatial asymmetries and supports the design\r\nof boundary-aware graph construction. Additional evaluations using\r\nIntegrated Forecasting System (IFS) and PanGu-Weather forecasts further\r\ndemonstrate that the model maintains high performance across different\r\ngridded data sources without retraining, highlighting its flexibility\r\nand potential to incorporate other AI-based meteorological models\r\nfor adaptable and effective air quality forecasting. These findings\r\nunderscore the potential of the proposed framework to serve as a computationally\r\nefficient and operationally feasible alternative to conventional chemical\r\ntransport models in future air quality management systems, particularly\r\nfor early warning systems and targeted emission control strategies.</p>","PeriodicalId":100230,"journal":{"name":"Chem & Bio Engineering","volume":"3 2","pages":"219–230"},"PeriodicalIF":8.4000,"publicationDate":"2026-02-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chem & Bio Engineering","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/cbe.5c00074","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/12/9 0:00:00","PubModel":"Epub","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
Abstract
Accurate forecasting of PM2.5 concentrations
is vital
for effective air quality management and public health protection,
particularly in the context of medium- to long-term planning. Such
forecasts are also essential for guiding emission control and timely
responses in urban and regional environments. Reliable prediction
over extended horizons critically depends on access to accurate, high-resolution
meteorological fields. To address limitations in traditional approaches
that rely on short-term site-level observations or retrospective meteorological
fields, this study proposes a deep learning framework that couples
AI-based gridded meteorological forecasts with a dynamic graph-based
architecture for PM2.5 prediction. The model captures evolving
spatiotemporal patterns of pollutant transport and enables extended-range
forecasts. By leveraging gridded meteorological forecasts, the proposed
framework reduces 3-day RMSE and MAE of the prediction by 12% compared
to models without the gridded inputs. For seasonal 10-day forecasts,
errors can be decreased by approximately 20% relative to the physics-based
Weather Research and Forecasting (WRF)-Community Multiscale Air Quality
(CMAQ) system. Furthermore, interpretability analysis reveals the
importance of wind-driven spatial asymmetries and supports the design
of boundary-aware graph construction. Additional evaluations using
Integrated Forecasting System (IFS) and PanGu-Weather forecasts further
demonstrate that the model maintains high performance across different
gridded data sources without retraining, highlighting its flexibility
and potential to incorporate other AI-based meteorological models
for adaptable and effective air quality forecasting. These findings
underscore the potential of the proposed framework to serve as a computationally
efficient and operationally feasible alternative to conventional chemical
transport models in future air quality management systems, particularly
for early warning systems and targeted emission control strategies.