{"title":"Numerical simulation of viscous fingering in CO₂ storage: Addressing the limitations of laboratory-derived relative permeabilities","authors":"S.A. Larki , A. Skauge , K.S. Sorbie , E.J. Mackay","doi":"10.1016/j.ijggc.2025.104523","DOIUrl":null,"url":null,"abstract":"<div><div>Gas injection in CCS is an unstable displacement process due to the viscosity contrast between injected gas and in-situ brine, a fact often overlooked in CO₂ storage modelling. Most studies estimating relative permeability (Relperms) for CCS rely on conventional methods. This paper applies a novel approach that explicitly considers viscous instability from injecting low-viscosity gas into more viscous brine. Based on our earlier studies (A. Beteta et al., 2024; Sorbie et al., 2020). viscous fingering is expected under viscous-dominated conditions. While strong capillary forces may suppress fingering at lab scale, the balance of viscous and capillary forces can shift at field scale, leading to pronounced gas fingering.</div><div>To model CO₂ injection, we used published CO₂/water Relperms from CCS experiments. Two approaches were compared: conventional Relperms estimation and an alternative viscous fingering-based method. Simulations using conventional CO₂/water Relperms showed no fingering patterns, whereas our earlier study indicated that core flood experiments with a water–CO₂ viscosity ratio of ∼55 may generate gas fingers. The second approach, based on maximum mobility, produced gas fingers and matched production and differential pressure equally well.</div><div>This apparent absence of fingering may suggest limitations in the conventional representation of flow dynamics under such conditions. Possible reasons why experimental relative permeabilities do not capture the expected “fingering behaviour” are discussed in this paper. The main difference between our proposed Relperms and lab derived Relperms is in the total mobility, with our Relperms having a higher total mobility at the shock front gas saturations (S<sub>gf</sub>) of CO<sub>2</sub>.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"148 ","pages":"Article 104523"},"PeriodicalIF":5.9000,"publicationDate":"2025-12-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"International Journal of Greenhouse Gas Control","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S175058362500221X","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/11/8 0:00:00","PubModel":"Epub","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0
Abstract
Gas injection in CCS is an unstable displacement process due to the viscosity contrast between injected gas and in-situ brine, a fact often overlooked in CO₂ storage modelling. Most studies estimating relative permeability (Relperms) for CCS rely on conventional methods. This paper applies a novel approach that explicitly considers viscous instability from injecting low-viscosity gas into more viscous brine. Based on our earlier studies (A. Beteta et al., 2024; Sorbie et al., 2020). viscous fingering is expected under viscous-dominated conditions. While strong capillary forces may suppress fingering at lab scale, the balance of viscous and capillary forces can shift at field scale, leading to pronounced gas fingering.
To model CO₂ injection, we used published CO₂/water Relperms from CCS experiments. Two approaches were compared: conventional Relperms estimation and an alternative viscous fingering-based method. Simulations using conventional CO₂/water Relperms showed no fingering patterns, whereas our earlier study indicated that core flood experiments with a water–CO₂ viscosity ratio of ∼55 may generate gas fingers. The second approach, based on maximum mobility, produced gas fingers and matched production and differential pressure equally well.
This apparent absence of fingering may suggest limitations in the conventional representation of flow dynamics under such conditions. Possible reasons why experimental relative permeabilities do not capture the expected “fingering behaviour” are discussed in this paper. The main difference between our proposed Relperms and lab derived Relperms is in the total mobility, with our Relperms having a higher total mobility at the shock front gas saturations (Sgf) of CO2.
由于注入气体和原位盐水之间的粘度差异,CCS中的注气是一个不稳定的驱油过程,这一事实在CO₂储存建模中经常被忽视。大多数估算CCS相对渗透率(Relperms)的研究都依赖于传统方法。本文采用了一种新颖的方法,明确考虑了将低粘度气体注入黏度更高的盐水所产生的黏性不稳定性。基于我们早期的研究(A. beta et al., 2024; Sorbie et al., 2020)。粘性指法是预期在粘性主导的条件下。虽然在实验室尺度上,强大的毛细力可能会抑制指动,但在现场尺度上,粘性和毛细力的平衡可能会发生变化,导致明显的气指动。为了模拟二氧化碳的注入,我们使用了CCS实验中公布的二氧化碳/水浓度。比较了两种方法:常规的Relperms估计方法和基于粘性指法的替代方法。使用常规CO 2 /water Relperms进行的模拟没有显示出指状模式,而我们早期的研究表明,水- CO 2粘度比为~ 55的岩心注水实验可能会产生气指状模式。第二种方法基于最大的流动性,产生了气指,同时也很好地匹配了产量和压差。这种明显的指法缺失可能表明在这种条件下流动动力学的传统表示存在局限性。可能的原因,为什么实验相对渗透率不捕获预期的“指法行为”在本文中进行了讨论。我们提出的Relperms和实验室衍生的Relperms之间的主要区别在于总迁移率,我们的Relperms在CO2的激波前气体饱和度(Sgf)下具有更高的总迁移率。
期刊介绍:
The International Journal of Greenhouse Gas Control is a peer reviewed journal focusing on scientific and engineering developments in greenhouse gas control through capture and storage at large stationary emitters in the power sector and in other major resource, manufacturing and production industries. The Journal covers all greenhouse gas emissions within the power and industrial sectors, and comprises both technical and non-technical related literature in one volume. Original research, review and comments papers are included.