Assessing PM2.5 pollution in the Northeastern United States from the 2023 Canadian wildfire smoke: an episodic study integrating air quality and health impact modeling with emissions and meteorological uncertainty analysis.

IF 5.6 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Environmental Research Letters Pub Date : 2025-11-01 Epub Date: 2025-10-17 DOI:10.1088/1748-9326/ae10c9
Hao He, Timothy P Canty, Russell R Dickerson, Joel Dreessen, Amir Sapkota, Michel Boudreaux
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引用次数: 0

Abstract

Between June 6 and 8, 2023, wildfires in Quebec, Canada generated massive smoke plumes that traveled long distances and deteriorated air quality across the Northeastern United States (US). Surface daily PM2.5 observations exceeded 100 µg m-3, affecting major cities such as New York City and Philadelphia, while many areas lacked PM2.5 monitors, making it difficult to assess local air quality conditions. To address this gap, we developed a WRF-CMAQ-BenMAP modeling system to provide rapid, spatially continuous estimates of wildfire-attributable PM2.5 concentrations and associated health impacts, particularly benefiting regions lacking air quality monitoring. CMAQ simulations driven by two wildfire emissions datasets and two meteorological drivers showed good agreement with PM2.5 observations, with linear regression results of R2 ∼0.6 and slope ∼0.9. We further quantified uncertainties introduced by varying emissions and meteorological drivers and found the choice of wildfire emissions dataset alone can alter PM2.5 simulations by up to 40 µg m-3 (∼40%). Short-term health impacts were evaluated using the BenMAP model. Validation against asthma-associated emergency department (ED) visits in New York State confirmed the framework's ability to replicate real-world outcomes, with ED visits increased up to ∼40%. The modeling results identified counties most severely affected by wildfire plumes, the majority of which lack regulatory air quality monitors. Our approach highlights the value of integrated modeling for identifying vulnerable populations and delivering timely health burden estimates, regardless of local monitoring availability.

从2023年加拿大野火烟雾中评估美国东北部的PM2.5污染:一项将空气质量和健康影响模型与排放和气象不确定性分析相结合的偶发研究。
在2023年6月6日至8日期间,加拿大魁北克的野火产生了大量的烟雾,这些烟雾传播了很长一段距离,并恶化了美国东北部的空气质量。地面每日PM2.5观测值超过100µg -3,影响到纽约市和费城等主要城市,而许多地区没有PM2.5监测仪,使当地空气质量状况难以评估。为了解决这一差距,我们开发了WRF-CMAQ-BenMAP建模系统,以提供野火导致的PM2.5浓度及其相关健康影响的快速、空间连续估计,特别是有利于缺乏空气质量监测的地区。由两个野火排放数据集和两个气象驱动因素驱动的CMAQ模拟结果与PM2.5观测值吻合良好,线性回归结果R2 ~ 0.6,斜率~ 0.9。我们进一步量化了不同排放和气象驱动因素带来的不确定性,发现仅野火排放数据集的选择就可以将PM2.5模拟值改变40µg -3(约40%)。使用BenMAP模型评估短期健康影响。对纽约州哮喘相关急诊科(ED)就诊的验证证实了该框架能够复制现实世界的结果,急诊科就诊增加了约40%。建模结果确定了受野火羽流影响最严重的县,其中大多数缺乏监管空气质量监测仪。我们的方法强调了综合建模在识别弱势群体和及时提供健康负担估计方面的价值,而不管当地是否有监测。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Environmental Research Letters
Environmental Research Letters 环境科学-环境科学
CiteScore
11.90
自引率
4.50%
发文量
763
审稿时长
4.3 months
期刊介绍: Environmental Research Letters (ERL) is a high-impact, open-access journal intended to be the meeting place of the research and policy communities concerned with environmental change and management. The journal''s coverage reflects the increasingly interdisciplinary nature of environmental science, recognizing the wide-ranging contributions to the development of methods, tools and evaluation strategies relevant to the field. Submissions from across all components of the Earth system, i.e. land, atmosphere, cryosphere, biosphere and hydrosphere, and exchanges between these components are welcome.
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