Benchmarking greenhouse gas emissions from US wastewater treatment for targeted reduction

IF 24.1
Sahar H. El Abbadi, Jianan Feng, Abigayle R. Hodson, Maryam Amouamouha, Margaret M. Busse, Christina Polcuch, Pengxiao Zhou, Jordan Macknick, Jeremy S. Guest, Jennifer R. Stokes-Draut, Jennifer B. Dunn
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Abstract

Here, to assess the national climate impact of wastewater treatment and inform decarbonization, we assembled a comprehensive greenhouse gas inventory of 15,863 facilities in the contiguous USA. Considering location and treatment configurations, we modelled on-site CH4, N2O and CO2 production and emissions associated with energy, chemical inputs and solids disposal. Using Monte Carlo simulations, we estimated median national emissions at 47 million tonnes of CO2 equivalent per year, with on-site process CH4 and N2O emissions exceeding current government estimates by 41%. Treatment configurations with anaerobic digesters are responsible for 16 million tonnes of CO2 equivalent per year of fugitive methane, outweighing benefits achieved through on-site electricity generation. Systems designed for nutrient removal have the highest greenhouse gas emissions intensity, attributable to energy requirements and N2O production, demonstrating current trade-offs between meeting water quality and climate objectives. We analysed key sensitivities and included a geospatial analysis to highlight the scale and distribution of opportunities for reducing life cycle greenhouse gas emissions. Benchmarking greenhouse gas emissions from wastewater treatment plants is an essential step in developing mitigation strategies. This is now achieved for the USA by modelling over 15,000 facilities using Monte Carlo simulations to obtain a national baseline.

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对美国废水处理的温室气体排放进行基准测试,以实现有针对性的减排
在这里,为了评估污水处理对国家气候的影响并为脱碳提供信息,我们收集了美国本土15863个设施的温室气体清单。考虑到地点和处理配置,我们模拟了与能源、化学投入和固体处置相关的现场CH4、N2O和CO2的产生和排放。通过蒙特卡罗模拟,我们估计全国每年的排放量中位数为4700万吨二氧化碳当量,现场过程中CH4和N2O的排放量比目前政府估计的高出41%。厌氧消化器的处理配置每年产生1600万吨二氧化碳当量的逸散甲烷,超过了现场发电所带来的效益。由于能源需求和N2O的产生,为去除营养物而设计的系统具有最高的温室气体排放强度,这表明了当前在满足水质和气候目标之间的权衡。我们分析了关键的敏感性,并纳入了地理空间分析,以突出减少生命周期温室气体排放的机会的规模和分布。制定污水处理厂温室气体排放基准是制定缓解战略的一个重要步骤。现在,美国通过使用蒙特卡罗模拟对15,000多个设施进行建模来获得国家基线,从而实现了这一目标。
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