Peng Liu, Yuanhang Li, Dong An, Shanshan Guan, Daishuang Zhang, Ning Tang, Hui Li, Yaxin Gu, Xiangyu Li, Yunwu Yu, Yaqi Wang
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引用次数: 0
Abstract
In this study, we developed a novel strain-sensing polyacrylamide (PAM) and sodium alginate (SA)/Cellulose/Pectin-Ca2+ (PSCP-Ca2+) composite hydrogel by integrating cellulose-pectin reinforcing networks into a dual-network matrix composed of PAM and SA, with Ca2+ ions serving as both structural cross-linkers and charge carriers. The PSCP-Ca2+ hydrogel demonstrated excellent mechanical properties (630 kPa stress, 1700% strain, and 5.8 MJ/m3 toughness), good self-healing properties, and high electrical conductivity (0.89 S/m). When employed as a flexible strain sensor, it exhibited a high gauge factor in both tension (GF = 3.74) and compression (GF = 6.48), a broad response range (0-1000% strain), and excellent fatigue resistance (2000+ tensile cycles and 500+ compressive cycles). This work provides valuable insights for designing high-performance hydrogel sensors and advances the practical implementation of flexible electronics in smart wearable devices and intelligent transportation systems.
期刊介绍:
Biomacromolecules is a leading forum for the dissemination of cutting-edge research at the interface of polymer science and biology. Submissions to Biomacromolecules should contain strong elements of innovation in terms of macromolecular design, synthesis and characterization, or in the application of polymer materials to biology and medicine.
Topics covered by Biomacromolecules include, but are not exclusively limited to: sustainable polymers, polymers based on natural and renewable resources, degradable polymers, polymer conjugates, polymeric drugs, polymers in biocatalysis, biomacromolecular assembly, biomimetic polymers, polymer-biomineral hybrids, biomimetic-polymer processing, polymer recycling, bioactive polymer surfaces, original polymer design for biomedical applications such as immunotherapy, drug delivery, gene delivery, antimicrobial applications, diagnostic imaging and biosensing, polymers in tissue engineering and regenerative medicine, polymeric scaffolds and hydrogels for cell culture and delivery.