Viscosity of Hydrogen-Enriched Natural Gas Blends (xH2 = 0, 5, 20, 50, and 80%) from 223 to 323 K and up to 30 MPa

IF 2.1 3区 工程技术 Q3 CHEMISTRY, MULTIDISCIPLINARY
Friday Junior Owuna, , , Antonin Chapoy*, , , Pezhman Ahmadi, , and , Rod Burgass, 
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引用次数: 0

Abstract

Natural gas (NG) transmission networks have been recognized as a cost-effective strategy for the distribution of hydrogen (H2). Thermophysical properties of H2-enriched NG are critical to the design and operations of these mixtures. Viscosities of H2-enriched NG mixtures (with H2 mol % values of 0, 5, 20, 50, and 80) were measured at temperatures from 223 to 323 K and pressures up to 30 MPa using a capillary tube viscometer. The measured viscosity data were evaluated against the predictions of a residual entropy scaling (SRES) method, the corresponding states using molecular dynamic simulations of Lennard-Jones fluids, a one-fluid reference corresponding states model (Pedersen), and an extended corresponding state SUPERTRAPP model. All the models were adequate for predicting the measured viscosities. This work contributes accurate viscosity data for H2-enriched NG blends and enhances the understanding of the blends’ properties, which enable modification to the NG distribution facilities to accommodate H2 transportation.

富氢天然气混合物(xH2 = 0,5,20,50和80%)的粘度从223到323 K,高达30 MPa
天然气(NG)传输网络已被认为是一种具有成本效益的氢气(H2)分配策略。富h2天然气的热物理性质对这些混合物的设计和操作至关重要。在223 ~ 323 K的温度和30 MPa的压力下,用毛细管粘度计测量了富H2的NG混合物(H2 mol %值分别为0、5、20、50和80)的粘度。根据剩余熵标度法(SRES)的预测、Lennard-Jones流体的分子动力学模拟、单流体参考对应状态模型(Pedersen)和扩展对应状态SUPERTRAPP模型,对测量的粘度数据进行了评估。所有的模型都足以预测所测粘度。这项工作为富含H2的天然气共混物提供了准确的粘度数据,增强了对共混物性质的理解,从而可以对天然气分配设施进行修改,以适应H2的输送。
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来源期刊
Journal of Chemical & Engineering Data
Journal of Chemical & Engineering Data 工程技术-工程:化工
CiteScore
5.20
自引率
19.20%
发文量
324
审稿时长
2.2 months
期刊介绍: The Journal of Chemical & Engineering Data is a monthly journal devoted to the publication of data obtained from both experiment and computation, which are viewed as complementary. It is the only American Chemical Society journal primarily concerned with articles containing data on the phase behavior and the physical, thermodynamic, and transport properties of well-defined materials, including complex mixtures of known compositions. While environmental and biological samples are of interest, their compositions must be known and reproducible. As a result, adsorption on natural product materials does not generally fit within the scope of Journal of Chemical & Engineering Data.
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