Characterization of a novel, large volume CdZnTe detector for marine applications.

IF 1.8 3区 工程技术 Q3 CHEMISTRY, INORGANIC & NUCLEAR
Georgios Siltzovalis, Varvara Lagaki, Ioannis Madesis, Theo J Mertzimekis
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Abstract

A large-volume (4 cm3) monolithic CdZnTe detector was selected for a novel underwater γ-radiation sensing instrument for radioactivity measurements near the seabed. The focus of this paper was to characterize the detector to adapt to the challenges expected during underwater operation. Initially, its efficiency and energy resolution were determined experimentally. Then, two underwater laboratory experiments were utilized. The first compared the detector efficiency from measurements performed in the air and then underwater. A decrease in efficiency was observed for low energy γ-rays during the underwater measurement. The second experiment evaluated the sensitivity of the method in underwater detection of 40K. The results revealed the limitations of the detector in real-life measurement scenarios. Next, Monte Carlo simulations were performed, focusing on the marinization of the detector. Candidate materials were investigated for the manufacturing of the necessary underwater housing. From the analysis of the results and considering real-world challenges expected in the marine environment, an aluminum housing was found to be optimal for the instrument development. Finally, the most efficient placement of the instrument with regard to the surface of the seabed was determined considering the detection range and the efficiency of the setup. It was concluded that a horizontal placement was the most suitable one. The proposed CdZnTe instrument is expected to provide a novel solution for underwater radioactivity studies in deep ocean environments and operation under harsh conditions. The main advantages it can offer are: the good energy resolution and efficiency, which are necessary for efficient underwater radioactivity monitoring.

一种新型的,大体积的用于海洋应用的CdZnTe探测器的特性。
采用大体积(4 cm3)单片CdZnTe探测器作为新型水下γ辐射传感仪器,用于海底附近的放射性测量。本文的重点是对探测器进行表征,以适应水下作业中预期的挑战。首先,通过实验确定了它的效率和能量分辨率。然后,利用两个水下实验室实验。第一项研究比较了探测器在空中和水下的测量效率。在水下测量时,观察到低能γ射线的效率下降。第二个实验评估了该方法在水下探测40K的灵敏度。结果揭示了探测器在实际测量场景中的局限性。接下来,进行了蒙特卡罗模拟,重点研究了探测器的海事化问题。研究了制造必要的水下壳体的候选材料。根据对结果的分析,并考虑到海洋环境中预期的现实挑战,发现铝制外壳是仪器开发的最佳选择。最后,考虑探测距离和设置效率,确定了仪器相对于海床表面的最有效放置位置。结果表明,水平放置是最合适的。所提出的CdZnTe仪器有望为深海环境和恶劣条件下的水下放射性研究提供新的解决方案。它的主要优点是:良好的能量分辨率和效率,这是有效监测水下放射性的必要条件。
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来源期刊
Applied Radiation and Isotopes
Applied Radiation and Isotopes 工程技术-核科学技术
CiteScore
3.00
自引率
12.50%
发文量
406
审稿时长
13.5 months
期刊介绍: Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.
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