The correlation between optical, mechanical, and radiation shielding properties for SiO2–ZnO–PbO2 glass samples doped with different concentrations of Gd2O3

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL
M.H.A. Mhareb , M.I. Sayyed , Awatif Alshamari , M. Kh Hamad
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Abstract

Four silicate glasses modified with ZnO and PbO2 and doped with different ratios of Gd2O3 were manufactured to evaluate their optical, mechanical, and radiation shielding characteristics. The evaluation used the Makishima–Mackenzie principle to assess the mechanical features, the absorption spectra to compute the band gap and optical features, and the Phy-X program for the estimation of the radiation shielding parameters. There was a 56.035 to 54.913 GPa modulus reduction with increased Gd2O3 and PbO2. Also, the band gap showed a reduction from 2.920 to 2.789 eV. The mechanical and optical properties results showed decreased glass stability with the addition of Gd2O3 and PbO2. On the other side, the radiation shielding behavior increased. For example, at 0.015 the mass attenuation coefficient increased from 74.974 to 78.600 cm2/g. According to the above results, it can be deduced that the present samples showed acceptable glass stability and radiation shielding parameters, nominating the glass for use as radiation shielding materials.
掺杂不同浓度Gd2O3的SiO2-ZnO-PbO2玻璃样品的光学、机械和辐射屏蔽性能的相关性
制备了四种以ZnO和PbO2改性并掺杂不同比例Gd2O3的硅酸盐玻璃,以评估其光学、机械和辐射屏蔽特性。评估采用Makishima-Mackenzie原理评估机械特性,吸收光谱计算带隙和光学特性,Phy-X程序估计辐射屏蔽参数。随着Gd2O3和PbO2的增加,模量降低了56.035 ~ 54.913 GPa。带隙也从2.920 eV减小到2.789 eV。机械性能和光学性能结果表明,加入Gd2O3和PbO2后,玻璃稳定性降低。另一方面,辐射屏蔽性能增强。例如,在0.015时,质量衰减系数从74.974增加到78.600 cm2/g。根据以上结果可以推断,本样品具有良好的玻璃稳定性和辐射屏蔽参数,可作为辐射屏蔽材料使用。
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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