Erosion and clogging mitigation in sandstone reservoirs through microbial carbonate precipitation: A microfluidic study

IF 8.4 1区 工程技术 Q1 ENGINEERING, GEOLOGICAL
Yun Lu , Yuze Wang
{"title":"Erosion and clogging mitigation in sandstone reservoirs through microbial carbonate precipitation: A microfluidic study","authors":"Yun Lu ,&nbsp;Yuze Wang","doi":"10.1016/j.enggeo.2025.108375","DOIUrl":null,"url":null,"abstract":"<div><div>Erosion and clogging near CO<sub>2</sub> injection wells present significant challenges to reservoir stability and injectivity, especially in weakly consolidated sandstones containing carbonate minerals. In this study, microfluidic chips were used to construct synthetic porous media mimicking weakly cemented sandstone, followed by Microbially Induced Calcium Carbonate Precipitation (MICP) treatment to reinforce pore structure and improve resistance to acid-induced degradation. Systematic experiments were conducted under varying pH, flow rates, and treatment cycles to simulate CO<sub>2</sub>-induced acidic flow conditions. Results demonstrate that MICP significantly enhances erosion resistance by forming multiscale CaCO<sub>3</sub> networks through particle bridging and interfacial cementation. A size-dependent buffering effect is observed during crystal dissolution, where smaller crystals dissolve first, locally increasing pH and delaying damage to larger structures. MICP also mitigates clogging by forming permeable crystal bridges at pore throats, restricting coarse particle transport while maintaining flow paths. The extent of erosion and clogging is strongly correlated with the initial cementation volume (<span><math><msub><mi>V</mi><msub><mi>CaCO</mi><mn>3</mn></msub></msub><mo>/</mo><msub><mi>V</mi><mi>V</mi></msub></math></span>), showing a dual-threshold response: systems with ≥4 % CaCO<sub>3</sub> remain stable, while those with &lt;2 % rapidly destabilize. MICP treatment raises the critical flow threshold and reduces sensitivity to acid flow, demonstrating its potential to improve injectivity and long-term storage reliability in CO<sub>2</sub> reservoirs.</div></div>","PeriodicalId":11567,"journal":{"name":"Engineering Geology","volume":"358 ","pages":"Article 108375"},"PeriodicalIF":8.4000,"publicationDate":"2025-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Engineering Geology","FirstCategoryId":"89","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0013795225004715","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, GEOLOGICAL","Score":null,"Total":0}
引用次数: 0

Abstract

Erosion and clogging near CO2 injection wells present significant challenges to reservoir stability and injectivity, especially in weakly consolidated sandstones containing carbonate minerals. In this study, microfluidic chips were used to construct synthetic porous media mimicking weakly cemented sandstone, followed by Microbially Induced Calcium Carbonate Precipitation (MICP) treatment to reinforce pore structure and improve resistance to acid-induced degradation. Systematic experiments were conducted under varying pH, flow rates, and treatment cycles to simulate CO2-induced acidic flow conditions. Results demonstrate that MICP significantly enhances erosion resistance by forming multiscale CaCO3 networks through particle bridging and interfacial cementation. A size-dependent buffering effect is observed during crystal dissolution, where smaller crystals dissolve first, locally increasing pH and delaying damage to larger structures. MICP also mitigates clogging by forming permeable crystal bridges at pore throats, restricting coarse particle transport while maintaining flow paths. The extent of erosion and clogging is strongly correlated with the initial cementation volume (VCaCO3/VV), showing a dual-threshold response: systems with ≥4 % CaCO3 remain stable, while those with <2 % rapidly destabilize. MICP treatment raises the critical flow threshold and reduces sensitivity to acid flow, demonstrating its potential to improve injectivity and long-term storage reliability in CO2 reservoirs.
通过微生物碳酸盐沉淀缓解砂岩储层的侵蚀和堵塞:微流体研究
注二氧化碳井附近的侵蚀和堵塞对储层的稳定性和注入能力构成了重大挑战,特别是在含碳酸盐矿物的弱胶结砂岩中。在本研究中,采用微流控芯片构建模拟弱胶结砂岩的合成多孔介质,然后采用微生物诱导碳酸钙沉淀(MICP)处理来强化孔隙结构,提高其抗酸降解能力。在不同的pH值、流速和处理周期下进行了系统的实验,以模拟二氧化碳诱导的酸性流动条件。结果表明,MICP通过颗粒桥接和界面胶结形成多尺度CaCO3网络,显著提高了耐蚀性。在晶体溶解过程中观察到一种与尺寸相关的缓冲效应,其中较小的晶体首先溶解,局部增加pH值并延迟对较大结构的破坏。MICP还通过在孔喉处形成可渗透的晶体桥来缓解堵塞,在保持流动路径的同时限制粗颗粒的传输。侵蚀和堵塞的程度与初始胶结体积(VCaCO3/VV)密切相关,表现出双阈值响应:CaCO3≥4%的体系保持稳定,而CaCO3≥2%的体系迅速不稳定。MICP处理提高了临界流量阈值,降低了对酸流的敏感性,显示了其提高二氧化碳储层注入能力和长期储存可靠性的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
Engineering Geology
Engineering Geology 地学-地球科学综合
CiteScore
13.70
自引率
12.20%
发文量
327
审稿时长
5.6 months
期刊介绍: Engineering Geology, an international interdisciplinary journal, serves as a bridge between earth sciences and engineering, focusing on geological and geotechnical engineering. It welcomes studies with relevance to engineering, environmental concerns, and safety, catering to engineering geologists with backgrounds in geology or civil/mining engineering. Topics include applied geomorphology, structural geology, geophysics, geochemistry, environmental geology, hydrogeology, land use planning, natural hazards, remote sensing, soil and rock mechanics, and applied geotechnical engineering. The journal provides a platform for research at the intersection of geology and engineering disciplines.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信