Integrated carbon capture and dry reforming of methane of mechanochemically synthesised dual-function materials

Abstract

Herein we report a green mechanochemical synthesis with low energy input of dual-function materials for integrated CO₂ capture and dry reforming of methane. The materials produced syngas during the CH₄ step (up to 0.6 mmol g⁻¹ CO and 7.7 mmol g⁻¹ H₂) and CO during the CO₂ step (up to 3.1 mmol g⁻¹) via the reverse Boudouard reaction due to the carbon produced from CH₄ cracking.