Purcell Effect in Epsilon-Near-Zero Microcavities

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
ACS Omega Pub Date : 2025-09-20 DOI:10.1021/acsomega.5c07448
Ali Panahpour*, , , Jussi Kelavuori, , and , Mikko Huttunen, 
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引用次数: 0

Abstract

Epsilon-near-zero (ENZ) photonics offers a compelling platform for integrated photonic systems, enabling a range of novel and extraordinary functionalities. However, the practical deployment of ENZ-based devices is constrained by high material losses and severe impedance mismatch, which are detrimental to applications requiring coherent light manipulation and efficient light-matter interaction. To address these challenges, we demonstrate that all-dielectric Bragg-reflection microcavities operated near their cutoff frequency, offer an ultralow-loss platform for enhancing light-matter interaction and exploring emission processes in the ENZ regime. While Bragg cavities are well-established, their potential as ENZ resonant microcavities remains largely unexplored. We investigate the Purcell effect and quality factor in these structures, comparing their performance with those of the perfect-electric-conductor and metallic counterparts. Through analytical derivations based on Fermi’s golden rule and field quantization in lossless dispersive media, we establish scaling laws that distinguish these ENZ cavities from conventional resonators. Frequency domain simulations validate our counterintuitive findings, demonstrating that in all-dielectric ENZ Bragg-reflection microcavities, the Purcell and quality factors scale as L0 and (L0)3, respectively, where L is the cavity length and λ0 is the resonance wavelength. Our results offer key insights into the design of ENZ-based photonic systems, paving the way for enhanced light-matter interactions in nonlinear optics and quantum photonics.

epsilon -近零微腔中的Purcell效应
epsilon -近零(ENZ)光子学为集成光子系统提供了一个引人注目的平台,实现了一系列新颖而非凡的功能。然而,基于enz的器件的实际部署受到高材料损耗和严重阻抗失配的限制,这不利于需要相干光操作和有效光-物质相互作用的应用。为了解决这些挑战,我们证明了全介质布拉格反射微腔在其截止频率附近工作,为增强光-物质相互作用和探索ENZ状态下的发射过程提供了一个超低损耗平台。虽然布拉格空腔已经得到了证实,但它们作为ENZ谐振微腔的潜力在很大程度上仍未被探索。我们研究了这些结构中的珀塞尔效应和质量因子,并将它们的性能与完美电导体和金属导体的性能进行了比较。通过基于费米黄金法则的解析推导和无损色散介质中的场量子化,我们建立了区分这些ENZ腔与传统谐振腔的标度定律。频域模拟验证了我们的反直觉发现,表明在全介质ENZ bragg反射微腔中,Purcell因子和质量因子分别为L/λ0和(L/λ0)3,其中L为腔长,λ0为共振波长。我们的研究结果为基于enz的光子系统的设计提供了关键的见解,为非线性光学和量子光子学中增强光-物质相互作用铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
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